[QE-users] Cholesky Decomposition Error

Giuseppe Mattioli giuseppe.mattioli at ism.cnr.it
Tue Jul 16 16:44:47 CEST 2024


Dear Antoine

    DESCRIPTION OF ITEMS:

       +--------------------------------------------------------------------
       Card's flags:   { alat | bohr | angstrom | crystal | crystal_sg }

       Default:        (DEPRECATED) alat
       Description:
                       Units for ATOMIC_POSITIONS:

                       alat :
                            atomic positions are in cartesian coordinates, in
                            units of the lattice parameter (either celldm(1)
                            or A). If no option is specified, 'alat'  
is assumed;
                            not specifying units is DEPRECATED and will no
                            longer be allowed in the future

You have not specified the units of ATOMIC_POSITIONS, so pw.x is using  
the default alat units. I suppose that you have provided crystal units  
instead, and this should be the source of the cholesky decomposition  
error, which 99% of times appears because of wrong coordinates.

HTH
Giuseppe


Quoting Antoine Moats <amoats at usc.edu>:

> Hello,
>
> I am trying to perform a scf calculation for a high entropy oxide, but I
> keep running into the following error:
>
> Error in routine  pdpotrf (1):
> problems computing cholesky decomposition
>
> I have tried a couple of things to no avail:
> -Increasing the ecutwfc to 75
> -Changing the diagonalization to cg
> -Making my own PAW pseudopotentials using the PBE solver
> -Replacing Eu with other elements
>
> Do you have any ideas as to what the issues could be? The structure was
> relaxed in VASP, so my thought process is simply that the positions are
> "bad"/result in a rounding error within the numerical techniques used by
> QE. If this is the case, what is the fix? Thanks!
>
> Antoine Moats
> Undergraduate
> University of Southern California/University of Tennesse, Knoxville
>
> Here is my code:
>
>   1 &CONTROL
>   2  calculation = 'scf'
>   3  prefix = 'HEO'
>   4  outdir = 'data'
>   5  verbosity = 'high'
>   6  pseudo_dir = 'pseudopotentials'
>   7  etot_conv_thr = 1.0D-6
>   8  forc_conv_thr = 1.0D-2
>   9  max_seconds = 1.0D7  ! default value (potentially change in the future
> for long calcs)
>  10 /
>  11
>  12 &SYSTEM
>  13  ecutrho = 600  ! guess
>  14  ecutwfc = 45   ! guess
>  15  ibrav = 0      ! see quantum espresso documentation
>  16  nat = 200      ! total number of atoms
>  17  ntyp = 7      ! total number of types of atoms
>  18  A = 1          ! lattice parameter (already incorporated into cell
> parameters)
>  19  occupations = 'smearing'
>  20  degauss = 0.01
>  21  nosym = .TRUE.
>  22 /
>  23
>  24 &ELECTRONS
>  25 diagonalization = 'cg'
>  26 diago_david_ndim = 8
>  27 /
>  28
>  29 &IONS
>  30 /
>  31
>  32 ATOMIC_SPECIES
>  33 Eu 151.964 Eu.pbe-spdn-kjpaw_psl.1.0.0.UPF
>  34 Sc 44.9559 Sc.pbe-spn-kjpaw_psl.1.0.0.UPF
>  35 Al 26.9813 Al.pbe-n-kjpaw_psl.1.0.0.UPF
>  36 Cr 51.9961 Cr.pbe-spn-kjpaw_psl.1.0.0.UPF
>  37 Fe 55.845  Fe.pbe-spn-kjpaw_psl.1.0.0.UPF
>  38 Ni 58.6934 Ni.pbe-spn-kjpaw_psl.1.0.0.UPF
>  39 O  15.999   O.pbe-n-kjpaw_psl.1.0.0.UPF
>  40
>  41 ATOMIC_POSITIONS
>  42 Eu 0.1131803489508531  0.9757807110698096  0.4948430002973888
>  43 Eu 0.3105561026392654  0.3777469985119398  0.4977522258180569
>  44 Eu 0.5104953473322690  0.7698372949819583  0.5075525147164309
>  45 Eu 0.7123579578802758  0.1700225065898888  0.4869360381636212
>  46 Eu 0.9077313977638648  0.5765461277747672  0.4939673548342658
>  47 Eu 0.1167447091798221  0.9824653575170831  0.9804847967065894
>  48 Eu 0.3030882766263624  0.3731587131156608  0.9958648272703060
>  49 Eu 0.5129411637215289  0.7732458810073197  0.9826450255235640
>  50 Eu 0.7128406915443793  0.1717821032694611  0.9955882007694374
>  51 Eu 0.9058647880979659  0.5685440143980997  0.9874214128553925
>  52 Eu 0.4927366240831404  0.2222270209180404  0.0098754554940163
>  53 Eu 0.6868405248134424  0.6238817322236990  0.0033343277112997
>  54 Eu 0.8866790846559295  0.0327723031834186 -0.0028947017470236
>  55 Eu 0.0896769675729570  0.4184226940691690  0.0064671406570571
>  56 Eu 0.2958339711150417  0.8344981282519404  0.9865551132845195
>  57 Eu 0.4871521909552198  0.2316891831214444  0.5137688243702805
>  58 Eu 0.6889614166111881  0.6283077550188551  0.5102250972046408
>  59 Eu 0.8821643676611727  0.0272332653861050  0.5121257457023076
>  60 Eu 0.0977832587259641  0.4289107521951567  0.5147338298195525
>  61 Eu 0.2867555333037768  0.8246336027691556  0.5192117928952809
>  62 Eu 0.3824236953978692  0.0287936382785004  0.7449773091423122
>  63 Eu 0.5877000649683850  0.4289914440194800  0.7453156396303776
>  64 Eu 0.7868670839910225  0.8297483191758092  0.7399401346849308
>  65 Eu 0.9888766764695095  0.2227684085093881  0.7466872572553094
>  66 Eu 0.1939219531169092  0.6285138366487760  0.7396199277460883
>  67 Eu 0.3897655981498755  0.0293205205956623  0.2324075928095888
>  68 Eu 0.5947933452330950  0.4207741390113546  0.2413173168554814
>  69 Eu 0.7904091093793340  0.8265324541315842  0.2469279962237142
>  70 Eu 0.9827904985063664  0.2236636780761965  0.2299587015973120
>  71 Eu 0.1906836735186699  0.6197414165015639  0.2498489060375883
>  72 Eu 0.2100120796198628  0.1743453482805615  0.7607811638813233
>  73 Eu 0.4108940774402721  0.5786430521073834  0.7629372001279854
>  74 Eu 0.6180721151892724  0.9733300569673395  0.7633321111844449
>  75 Eu 0.8096276456677156  0.3683278690919098  0.7674103492653521
>  76 Eu 0.0147894798964761  0.7783316807791938  0.7575030099115683
>  77 Eu 0.2047495457832584  0.1768404672524297  0.2477334811233753
>  78 Eu 0.4033620682094110  0.5674257994078140  0.2554052702391294
>  79 Eu 0.6177899902564712  0.9810230985001345  0.2586784091929746
>  80 Eu 0.8041435818595506  0.3665164128506184  0.2470468402009450
>  81 Eu 0.0143586537693693  0.7710663421650347  0.2596674342814461
>  82 Sc 0.9986229364647106 -0.0006524208809492  0.2490610375686294
>  83 Sc 0.4005847972477796  0.7995040767414829  0.2490144027479403
>  84 Sc 0.4005744790945042  0.2989106052671023  0.2507992525512067
>  85 Sc 0.5988762747603588  0.6992118396813013  0.2507137538972432
>  86 Sc 0.9987104886458006  0.4966264316921545  0.2504312702917976
>  87 Sc 0.8994558796273646  0.3024578798785276  0.5012115418408654
>  88 Sc 0.1015179150459481  0.7008354240821598  0.0032002602108944
>  89 Sc 0.5019216994784226  0.0009161296161020  0.5016526188730493
>  90 Al 0.0001580516609265 -0.0001655330093875  0.7483157042737832
>  91 Al 0.2031507047571995  0.4020045010285742  0.7503733951563001
>  92 Al 0.6016574235728038  0.6985093677074741  0.7498342319419380
>  93 Al 0.6976292377316944  0.8997827375291476  0.5027885875629107
>  94 Al 0.8991504209691372  0.2969276812951809  0.9956264925308195
>  95 Al 0.3042066872864854  0.6026229157458037  0.5021539776696030
>  96 Al 0.4986703531104243  0.0006588591477152 -0.0053580067835508
>  97 Al 0.6984503915775195  0.3973899905012958  0.9965105401979236
>  98 Cr 0.8001260031846013  0.5986686999818260  0.2474681754904098
>  99 Cr 0.2016708888094732  0.8988102754536414  0.2514156270904139
> 100 Cr 0.3982236884870458  0.3040728416548124  0.7543490371380014
> 101 Cr 0.0014896176210110  0.4992075381593036  0.7508446963039183
> 102 Cr 0.2991013061340603  0.1021403202906894  0.4945520729167415
> 103 Cr 0.4989479056326999  0.5042456346451089  0.5042698415526516
> 104 Cr 0.7012575163293637  0.8994962661670558  0.0035588092818000
> 105 Cr 0.1002460666822707  0.2023693001534271  0.4997238592060068
> 106 Fe 0.6010196417746179  0.1980870269729934  0.7499376807868765
> 107 Fe 0.7974649863565728  0.5998011689496410  0.7508339596556208
> 108 Fe 0.0999340111963343  0.6977444672344862  0.5045469061840486
> 109 Fe 0.5010962497730175  0.4957943806608978  0.0010802950620063
> 110 Fe 0.6972994091604469  0.3973924762586531  0.5057534407196219
> 111 Fe 0.9012913178130821  0.8028350703337936  0.5029014124547415
> 112 Fe 0.9023025605163396  0.8023088055145375  0.9968753066453485
> 113 Fe 0.2986425571743697  0.5996094468430092  0.0001535744683252
> 114 Ni 0.1974362321784239  0.3979571547618609  0.2531453859627189
> 115 Ni 0.6016216451803531  0.1997266516720537  0.2485606781559177
> 116 Ni 0.4034032299811893  0.8023454046689175  0.7505760690148137
> 117 Ni 0.8006874223402385  0.1016449747452808  0.2495774053404509
> 118 Ni 0.1974992095425996  0.9041041880198774  0.7474829017776103
> 119 Ni 0.8006533301796352  0.0989360586075278  0.7488344866008355
> 120 Ni 0.3019115421658655  0.1011467754902807  0.9975313705421845
> 121 Ni 0.0964475729317619  0.1993548200397149  0.9951342498894407
> 122 O 0.1945187590851784  0.1398421348499920  0.0480751110881268
> 123 O 0.3932153689133333  0.5309987780166532  0.0481762693825505
> 124 O 0.5996394973617279  0.9331521064714866  0.0485514173981735
> 125 O 0.7942846392237017  0.3408301090871457  0.0381638113469535
> 126 O 0.9863182402471621  0.7298821314392165  0.0553105627641397
> 127 O 0.1932350424789405  0.1391636006190096  0.5515889691823576
> 128 O 0.3962802851467347  0.5408611490393264  0.5561438660420972
> 129 O 0.5961274135123740  0.9309792218250361  0.5581078469668437
> 130 O 0.7883301954286537  0.3365886795380312  0.5627981942912647
> 131 O 0.9931350412041157  0.7349943246834381  0.5542578068682307
> 132 O 0.3993367466062662  0.0718882427901716  0.4445883324021335
> 133 O 0.6006289563954444  0.4667184005196785  0.4517350934435356
> 134 O 0.8032680671043363  0.8603825644966326  0.4531378999786240
> 135 O 0.0151332926937110  0.2635443600660237  0.4498064429453581
> 136 O 0.2092501219428340  0.6584958226595227  0.4555736937261070
> 137 O 0.4103390031325591  0.0593772763855088  0.9442707535228796
> 138 O 0.6115001401461004  0.4609364662028251  0.9470952905060243
> 139 O 0.8036666965322581  0.8636313943903546  0.9466566098140619
> 140 O 0.0004753062971064  0.2647488666464351  0.9459606605807427
> 141 O 0.2128180924479490  0.6708740217666171  0.9419318588178134
> 142 O 0.3028476632594860  0.8689623720096176  0.3089625883171732
> 143 O 0.5086525587598270  0.2649593354500644  0.3104597458861026
> 144 O 0.7123454307921875  0.6601246816393606  0.3023698360688170
> 145 O 0.9060103255775327  0.0641877841354449  0.3084066944107813
> 146 O 0.1065466713493888  0.4618106273196617  0.3122635171397281
> 147 O 0.3070651650267187  0.8663778014552092  0.7905717986682990
> 148 O 0.4977172187719855  0.2694718905327103  0.8011707920595648
> 149 O 0.7031899781655157  0.6634746768612784  0.7970770831036676
> 150 O 0.9127420697519701  0.0583209218512878  0.7952874693961405
> 151 O 0.1067817177783779  0.4656967404784730  0.7972395515439520
> 152 O 0.2918011684547046  0.3376012238144009  0.1993558645814594
> 153 O 0.4892636141702166  0.7263041114217590  0.1882869307086155
> 154 O 0.6953142182787952  0.1370842377547587  0.1943165782598997
> 155 O 0.8857249566866442  0.5382550142751731  0.1953352054761023
> 156 O 0.1007571073422442  0.9334651183229357  0.1950301778883299
> 157 O 0.2948679435590675  0.3405755115765721  0.7022316821289608
> 158 O 0.5023266623227992  0.7351348499463858  0.7084014985545092
> 159 O 0.6895588223645293  0.1371369334067230  0.6956327004402413
> 160 O 0.8970055214656850  0.5308664161555869  0.7015498964145092
> 161 O 0.0862401004039534  0.9404533097093551  0.6951775140091364
> 162 O 0.0837551743900314  0.1103176246968863  0.3585049224038924
> 163 O 0.2825478069052377  0.5115176536585176  0.3665859164275551
> 164 O 0.4856105184719381  0.9111620079884440  0.3453040466099655
> 165 O 0.6831096759180036  0.3158091702219053  0.3553185347741569
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> 167 O 0.0783920211379794  0.1042579820060380  0.8403467899816532
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> 169 O 0.4893382268216454  0.9111132180062148  0.8614208417077482
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> 183 O 0.5676675485632604  0.5641722815801790  0.1446766276379610
> 184 O 0.7592481369570834  0.9617416737210599  0.1402830403022464
> 185 O 0.9552396767967103  0.3660076872348869  0.1378607165161261
> 186 O 0.1601514742210292  0.7675061687531893  0.1657354790891493
> 187 O 0.3593740302783414  0.1736821693616645  0.6463247402669599
> 188 O 0.5631838498336679  0.5723492700083296  0.6478935066070095
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> 191 O 0.1620821472044290  0.7703339828031849  0.6447339623369712
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> 201 O 0.3201800162354706  0.6844058501966240  0.6433071496779393
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> 206 O 0.0649954417540766  0.5676933736082134  0.6077143719132060
> 207 O 0.2624808209037562  0.9603220478466843  0.1115330520575724
> 208 O 0.4694487772391461  0.3697354911514922  0.1011923464192709
> 209 O 0.6674665099135744  0.7710445068255264  0.0996640803697750
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> 211 O 0.0683194569712264  0.5647914465222824  0.1016578457630088
> 212 O 0.4172463914640329  0.8893582530422841  0.5981540922916144
> 213 O 0.6136588857119518  0.2989515066475312  0.6086593915895356
> 214 O 0.8205437316394107  0.6896185626820118  0.6014357397538959
> 215 O 0.0231408867071053  0.0951568094431540  0.5959764541236864
> 216 O 0.2249369147253923  0.4882548273687719  0.6068683950476279
> 217 O 0.4210290365725239  0.8949059407418130  0.0917639155985315
> 218 O 0.6241823657409119  0.2977757012288595  0.0950144404570943
> 219 O 0.8137160426816573  0.6854426365119584  0.1088807957845803
> 220 O 0.0141514639703305  0.0920475201303485  0.0982703804874842
> 221 O 0.2196108087447415  0.4881031244770543  0.0955286859236969
> 222 O 0.1805664206871734  0.3157904830990086  0.8873095481744453
> 223 O 0.3823880557866521  0.7063922748073229  0.9030944934375937
> 224 O 0.5805112897035125  0.1079155078179337  0.9020085497146789
> 225 O 0.7770447687465338  0.5056419296861789  0.8983115658069324
> 226 O 0.9812984563292539  0.9077598194369444  0.8921900823200778
> 227 O 0.1799710270089699  0.3018345036917133  0.4113732097700553
> 228 O 0.3806522191722605  0.7035169451707672  0.4057438840018228
> 229 O 0.5857240053453263  0.1088497229890844  0.3987811164920322
> 230 O 0.7791781335343824  0.5150848901189575  0.3906058875955839
> 231 O 0.9840231252464969  0.8992032144301072  0.3987692502011514
> 232 O 0.3375436885131067  0.2381676066388068  0.8862282201381381
> 233 O 0.5434256281352697  0.6293606358858472  0.8933441940454255
> 234 O 0.7374868043648809  0.0259148956899109  0.9044778607790772
> 235 O 0.9375775038226563  0.4294413056367892  0.8956708451573859
> 236 O 0.1348063327897248  0.8326742006926851  0.8982407526791919
> 237 O 0.3303376959531669  0.2272775550651744  0.4071643550453899
> 238 O 0.5357876265989562  0.6277949891309575  0.4079573345364130
> 239 O 0.7355760652850561  0.0236554815563012  0.4074924485706826
> 240 O 0.9272090606933341  0.4343697201740280  0.3981539552492892
> 241 O 0.1418549373477760  0.8356170897081856  0.3945976980079966
> 242
> 243 K_POINTS gamma
> 244
> 245 CELL_PARAMETERS alat
> 246 -5.5801015826000011  -15.6405981208000018   -0.0000000000000000
> 247 -11.160203165200002    7.8202990604000009    0.0000000000000000
> 248 -0.0000000000000000   -0.0000000000000000  -11.0332000000000008



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E-mail: <giuseppe.mattioli at ism.cnr.it>



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