[QE-users] Issues with vc-relax for a slab

Anupriya Nyayban anupriya_rs at phy.nits.ac.in
Fri Jan 26 11:28:53 CET 2024


Dear Dr. Chirantan Pramanik,

Thank you for the reply!
No, I haven't done vc-relax for a surface earlier but with relax also I am
facing a similar problem. However, I will try 'relax calculation' by
increasing the electron_maxstep.

with regards
Anupriya Nyayban
Postdoc, IIT Madras


On Fri, Jan 26, 2024 at 12:44 PM Anupriya Nyayban <
anupriya_rs at phy.nits.ac.in> wrote:

> Dear users and experts,
>
> I have considered a (311) plane of 2 layers of ZnFe2O4 structure. The
> attached input file is for the vc-relax calculation.
>
> &CONTROL
>   calculation='vc-relax'
>   restart_mode='from_scratch',
>   prefix='zn'
>   pseudo_dir = '.'
>   outdir='tmp'
>   verbosity='high'
>   etot_conv_thr = 1.0D-5
>   forc_conv_thr = 1.0D-4
> /
> &SYSTEM
>   ibrav = 0
>   A =   21.62370
>   nat = 112
>   ntyp = 3
>   ecutwfc = 30.0,
>   ecutrho = 240.0,
>   occupations = 'smearing',
>   smearing = 'mv',
>   degauss = 0.02,
>   vdw_corr  = 'DFT-D3'
> /
> &ELECTRONS
>    conv_thr =  1.d-9
>    mixing_beta = 0.3
>   electron_maxstep = 300
>   startingpot = "atomic"
>   startingwfc = "atomic+random"
> /
> &IONS
>   ion_dynamics = "bfgs"
> /
> &CELL
>   cell_dynamics = "bfgs"
>   press_conv_thr = 5.00000e-01
> /
> CELL_PARAMETERS {alat}
>   1.000000000000000   0.000000000000000   0.000000000000000
>   0.299999977738132   0.331662474918549   0.000000000000000
>   0.000000000000000   0.000000000000000   2.019068156482969
> ATOMIC_SPECIES
>   Zn   65.38000  Zn_ONCV_PBE-1.0.upf
>   Fe   55.84500  Fe_ONCV_PBE-1.0.upf
>    O   15.99900  O_ONCV_PBE-1.0.upf
> ATOMIC_POSITIONS {crystal}
> Zn   0.863636000000000   0.954545000000000   0.475797000000000
> Zn   0.863636000000000   0.454545000000000   0.475797000000000
> Zn   0.363636000000000   0.454545000000000   0.475797000000000
> Zn   0.363636000000000   0.954545000000000   0.475797000000000
> Zn   0.545454000000000   0.181819000000000   0.487603000000000
> Zn   0.045455000000000   0.181818000000000   0.487603000000000
> Zn   0.045455000000000   0.681818000000000   0.487603000000000
> Zn   0.545455000000000   0.681818000000000   0.487602000000000
> Zn   0.590909000000000   0.863636000000000   0.523020000000000
> Zn   0.590909000000000   0.363636000000000   0.523020000000000
> Zn   0.090909000000000   0.363636000000000   0.523020000000000
> Zn   0.090909000000000   0.863636000000000   0.523020000000000
> Zn   0.272727000000000   0.090909000000000   0.534825000000000
> Zn   0.772727000000000   0.090909000000000   0.534826000000000
> Zn   0.772727000000000   0.590909000000000   0.534826000000000
> Zn   0.272727000000000   0.590909000000000   0.534825000000000
> Fe   0.954546000000000   0.068182000000000   0.481700000000000
> Fe   0.704545000000000   0.318182000000000   0.481700000000000
> Fe   0.204546000000000   0.568182000000000   0.481700000000000
> Fe   0.590909000000000   0.863636000000000   0.458088000000000
> Fe   0.204546000000000   0.818181000000000   0.481700000000000
> Fe   0.704545000000000   0.568182000000000   0.481700000000000
> Fe   0.590909000000000   0.363636000000000   0.458088000000000
> Fe   0.954545000000000   0.568182000000000   0.481700000000000
> Fe   0.704546000000000   0.818182000000000   0.481700000000000
> Fe   0.204545000000000   0.068182000000000   0.481700000000000
> Fe   0.204545000000000   0.318182000000000   0.481700000000000
> Fe   0.704546000000000   0.068181000000000   0.481700000000000
> Fe   0.454545000000000   0.068182000000000   0.481700000000000
> Fe   0.090909000000000   0.863637000000000   0.458088000000000
> Fe   0.090909000000000   0.363636000000000   0.458088000000000
> Fe   0.454545000000000   0.568182000000000   0.481700000000000
> Fe   0.681818000000000   0.977272000000000   0.528922000000000
> Fe   0.431818000000000   0.227273000000000   0.528922000000000
> Fe   0.931818000000000   0.477273000000000   0.528923000000000
> Fe   0.318182000000000   0.772727000000000   0.505311000000000
> Fe   0.931818000000000   0.727272000000000   0.528923000000000
> Fe   0.431818000000000   0.477273000000000   0.528922000000000
> Fe   0.318182000000000   0.272727000000000   0.505311000000000
> Fe   0.681818000000000   0.477273000000000   0.528923000000000
> Fe   0.431818000000000   0.727273000000000   0.528923000000000
> Fe   0.931818000000000   0.977273000000000   0.528923000000000
> Fe   0.931818000000000   0.227273000000000   0.528923000000000
> Fe   0.431818000000000   0.977272000000000   0.528923000000000
> Fe   0.181818000000000   0.977273000000000   0.528923000000000
> Fe   0.818182000000000   0.772728000000000   0.505311000000000
> Fe   0.818182000000000   0.272727000000000   0.505311000000000
> Fe   0.181818000000000   0.477273000000000   0.528923000000000
>  O   0.021208000000000   0.351541000000000   0.468710000000000
>  O   0.642439000000000   0.036341000000000   0.493900000000000
>  O   0.269690000000000   0.845466000000000   0.471866000000000
>  O   0.521208000000000   0.584834000000000   0.468711000000000
>  O   0.521208000000000   0.084834000000000   0.468710000000000
>  O   0.021208000000000   0.851541000000000   0.468710000000000
>  O   0.269690000000000   0.345466000000000   0.471866000000000
>  O   0.642439000000000   0.536342000000000   0.493900000000000
>  O   0.142439000000000   0.536342000000000   0.493900000000000
>  O   0.021208000000000   0.084834000000000   0.468710000000000
>  O   0.769690000000000   0.345466000000000   0.471866000000000
>  O   0.521208000000000   0.851541000000000   0.468711000000000
>  O   0.887883000000000   0.284822000000000   0.494689000000000
>  O   0.766652000000000   0.100022000000000   0.469499000000000
>  O   0.387883000000000   0.551530000000000   0.494689000000000
>  O   0.139401000000000   0.790898000000000   0.491533000000000
>  O   0.639401000000000   0.790898000000000   0.491533000000000
>  O   0.387883000000000   0.284822000000000   0.494689000000000
>  O   0.887883000000000   0.551530000000000   0.494689000000000
>  O   0.266652000000000   0.100022000000000   0.469499000000000
>  O   0.266652000000000   0.600022000000000   0.469499000000000
>  O   0.639401000000000   0.290898000000000   0.491533000000000
>  O   0.887882000000000   0.051530000000000   0.494689000000000
>  O   0.387883000000000   0.784822000000000   0.494689000000000
>  O   0.887883000000000   0.784822000000000   0.494689000000000
>  O   0.387883000000000   0.051530000000000   0.494689000000000
>  O   0.766652000000000   0.600022000000000   0.469499000000000
>  O   0.142439000000000   0.036341000000000   0.493900000000000
>  O   0.021208000000000   0.584834000000000   0.468710000000000
>  O   0.521209000000000   0.351541000000000   0.468710000000000
>  O   0.769690000000000   0.845466000000000   0.471866000000000
>  O   0.139401000000000   0.290898000000000   0.491533000000000
>  O   0.748481000000000   0.260632000000000   0.515933000000000
>  O   0.369712000000000   0.945432000000000   0.541123000000000
>  O   0.996962000000000   0.754557000000000   0.519089000000000
>  O   0.248481000000000   0.493925000000000   0.515933000000000
>  O   0.248481000000000   0.993924000000000   0.515933000000000
>  O   0.748481000000000   0.760632000000000   0.515933000000000
>  O   0.996962000000000   0.254556000000000   0.519089000000000
>  O   0.369712000000000   0.445432000000000   0.541123000000000
>  O   0.869712000000000   0.445433000000000   0.541123000000000
>  O   0.748481000000000   0.993924000000000   0.515933000000000
>  O   0.496962000000000   0.254556000000000   0.519089000000000
>  O   0.248481000000000   0.760632000000000   0.515933000000000
>  O   0.615155000000000   0.193913000000000   0.541912000000000
>  O   0.493924000000000   0.009113000000000   0.516722000000000
>  O   0.115155000000000   0.460621000000000   0.541912000000000
>  O   0.866674000000000   0.699989000000000   0.538756000000000
>  O   0.366674000000000   0.699989000000000   0.538756000000000
>  O   0.115155000000000   0.193913000000000   0.541912000000000
>  O   0.615155000000000   0.460621000000000   0.541912000000000
>  O   0.993924000000000   0.009113000000000   0.516722000000000
>  O   0.993924000000000   0.509113000000000   0.516722000000000
>  O   0.366674000000000   0.199989000000000   0.538756000000000
>  O   0.615155000000000   0.960621000000000   0.541912000000000
>  O   0.115155000000000   0.693913000000000   0.541912000000000
>  O   0.615155000000000   0.693913000000000   0.541912000000000
>  O   0.115155000000000   0.960621000000000   0.541912000000000
>  O   0.493924000000000   0.509113000000000   0.516722000000000
>  O   0.869712000000000   0.945432000000000   0.541123000000000
>  O   0.748481000000000   0.493925000000000   0.515933000000000
>  O   0.248481000000000   0.260632000000000   0.515933000000000
>  O   0.496962000000000   0.754557000000000   0.519089000000000
>  O   0.866674000000000   0.199989000000000   0.538756000000000
> K_POINTS {automatic}
>  2 2 1 1 1 1
>
> The following is how the energy changes after each optimization step. At
> the last optimization step ( Energy error = 1.5E+00 Ry), scf didn't
> converge even after 300 iterations.
>     Energy error            =      0.0E+00 Ry
>      Energy error            =      1.9E+01 Ry
>      Energy error            =      2.5E+01 Ry
>      Energy error            =      2.7E+01 Ry
>      Energy error            =      2.7E+01 Ry
>      Energy error            =      2.7E+01 Ry
>      Energy error            =      2.4E+01 Ry
>      Energy error            =      2.0E+01 Ry
>      Energy error            =      1.5E+01 Ry
>      Energy error            =      1.1E+01 Ry
>      Energy error            =      8.3E+00 Ry
>      Energy error            =      6.5E+00 Ry
>      Energy error            =      5.1E+00 Ry
>      Energy error            =      4.3E+00 Ry
>      Energy error            =      3.7E+00 Ry
>      Energy error            =      3.2E+00 Ry
>      Energy error            =      2.8E+00 Ry
>      Energy error            =      2.5E+00 Ry
>      Energy error            =      2.2E+00 Ry
>      Energy error            =      2.0E+00 Ry
>      Energy error            =      1.7E+00 Ry
>      Energy error            =      1.5E+00 Ry
> Please suggest how I can overcome the issue and what may be the reason! It
> will be really helpful!
>
>
> Thank you!
> Anupriya Nyayban
> Postdoc, IIT Madras
>
> On Wed, Jan 24, 2024 at 6:02 PM Anupriya Nyayban <
> anupriya_rs at phy.nits.ac.in> wrote:
>
>> Dear users and experts,
>>
>> I have considered a (311) plane of 2 layers of ZnFe2O4 structure. The
>> attached input file is for the vc-relax calculation. The following is how
>> the energy changes after each optimization step. At the last optimization
>> step ( Energy error = 1.5E+00 Ry), scf didn't converge even after 300
>> iterations.
>>     Energy error            =      0.0E+00 Ry
>>      Energy error            =      1.9E+01 Ry
>>      Energy error            =      2.5E+01 Ry
>>      Energy error            =      2.7E+01 Ry
>>      Energy error            =      2.7E+01 Ry
>>      Energy error            =      2.7E+01 Ry
>>      Energy error            =      2.4E+01 Ry
>>      Energy error            =      2.0E+01 Ry
>>      Energy error            =      1.5E+01 Ry
>>      Energy error            =      1.1E+01 Ry
>>      Energy error            =      8.3E+00 Ry
>>      Energy error            =      6.5E+00 Ry
>>      Energy error            =      5.1E+00 Ry
>>      Energy error            =      4.3E+00 Ry
>>      Energy error            =      3.7E+00 Ry
>>      Energy error            =      3.2E+00 Ry
>>      Energy error            =      2.8E+00 Ry
>>      Energy error            =      2.5E+00 Ry
>>      Energy error            =      2.2E+00 Ry
>>      Energy error            =      2.0E+00 Ry
>>      Energy error            =      1.7E+00 Ry
>>      Energy error            =      1.5E+00 Ry
>> Please suggest how I can overcome the issue and what may be the reason!
>>
>> Thank you!
>>
>> With regards
>> Anupriya Nyayban
>> IIT Madras, India
>>
>
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