[QE-users] Adsorption of molecules on the slab

khouini_f at znu.ac.ir khouini_f at znu.ac.ir
Fri Oct 7 21:26:41 CEST 2022


HiI am investigating the adsorption configuration of an organic molecule on platinum metal. When relaxing the molecule on the surface, after several steps, unfortunately, the structure of my molecule changes and actually breaks its bonds and the molecule loses its original structure.I have no idea how to solve this problem so that the structure of the molecule is fixed and only the configuration is optimized on the surface, any help would be great.My input file is belowThank you in advance
&CONTROL
        calculation   = "relax"
    restart_mode='from_scratch',
    prefix='.',
    pseudo_dir = '.',
    outdir='.',
                   verbosity = 'high' ,
                     tstress = .true. ,
                     tprnfor = .true. ,              
                      forc_conv_thr =   1.94469e-03
                       nstep=200
/
&SYSTEM
     ibrav                     = 0
    nat                       = 75
    nspin                     = 2
    ntyp                      = 4
     occupations= "smearing",
    smearing= 'methfessel-paxton',
    degauss=0.02,
    assume_isolated='2D',
    ecutwfc=30,
    ecutrho=240,
    starting_magnetization =  0.2
    nosym=.true.
/
&ELECTRONS
    conv_thr         =  1.00000e-07
    electron_maxstep = 300
    mixing_beta      =  3.00000e-01
    mixing_mode = "local-TF"
/
&IONS
    ion_dynamics = "bfgs"
/
K_POINTS {automatic}
 3  3  1  0 0 0
CELL_PARAMETERS {angstrom}
  10.922466325  -0.000000001   0.000000000
  -5.461233163   9.459132775   0.000000000
   0.000000000   0.000000000  18.000000000
ATOMIC_SPECIES
Pt    195.07800  pt_pbe_v1.4.uspp.F.UPF
 H    1.00784     H.pbe-rrkjus_psl.1.0.0.UPF
 O    15.999      O.pbe-n-kjpaw_psl.0.1.UPF
 C    12.0107     C.pbe-n-kjpaw_psl.1.0.0.UPF
ATOMIC_POSITIONS {angstrom}
Pt            0.0000077644        1.5765353552       16.3472430825
Pt            1.3653138403        0.7882699234       13.9807271384
Pt            0.0000000000        0.0000000000       11.6344210000    0   0   0
Pt           -0.0000000001        1.5765263758        9.3594310000    0   0   0
Pt           -1.3652992973        3.9413174027       16.3472432565
Pt            0.0000056911        3.1530542088       13.9807237385
Pt           -1.3653117209        2.3647890738       11.6344210000    0   0   0
Pt           -1.3653117210        3.9413154497        9.3594310000    0   0   0
Pt           -2.7306069919        6.3060985669       16.3472454145
Pt           -1.3653034692        5.5178371573       13.9807247039
Pt           -2.7306234418        4.7295791277       11.6344210000    0   0   0
Pt           -2.7306234419        6.3061045235        9.3594310000    0   0   0
Pt           -4.0959140592        8.6708836324       16.3472472241
Pt           -2.7306117082        7.8826191304       13.9807317397
Pt           -4.0959361427        7.0943682015       11.6344210000    0   0   0
Pt           -4.0959361428        8.6708945773        9.3594310000    0   0   0
Pt            2.7306236460        1.5765362703       16.3472408801
Pt            4.0959318247        0.7882691829       13.9807260288
Pt            2.7306234415       -0.0000000002       11.6344210000    0   0   0
Pt            2.7306234414        1.5765263756        9.3594310000    0   0   0
Pt            1.3653164814        3.9413181222       16.3472414781
Pt            2.7306235902        3.1530536188       13.9807225982
Pt            1.3653117206        2.3647890736       11.6344210000    0   0   0
Pt            1.3653117205        3.9413154495        9.3594310000    0   0   0
Pt            0.0000090139        6.3060992417       16.3472433990
Pt            1.3653145269        5.5178365556       13.9807237339
Pt           -0.0000000003        4.7295791275       11.6344210000    0   0   0
Pt           -0.0000000004        6.3061045233        9.3594310000    0   0   0
Pt           -1.3652981764        8.6708842497       16.3472450356
Pt            0.0000064858        7.8826185842       13.9807309194
Pt           -1.3653117212        7.0943682013       11.6344210000    0   0   0
Pt           -1.3653117213        8.6708945771        9.3594310000    0   0   0
Pt            5.4612372260        1.5765360174       16.3472433993
Pt            6.8265475346        0.7882704581       13.9807287820
Pt            5.4612478630       -0.0000000004       11.6344210000    0   0   0
Pt            5.4612478629        1.5765263755        9.3594310000    0   0   0
Pt            4.0959301298        3.9413179086       16.3472437141
Pt            5.4612392613        3.1530548263       13.9807252600
Pt            4.0959361421        2.3647890735       11.6344210000    0   0   0
Pt            4.0959361420        3.9413154493        9.3594310000    0   0   0
Pt            2.7306226904        6.3060990582       16.3472459231
Pt            4.0959300283        5.5178377680       13.9807261407
Pt            2.7306234412        4.7295791273       11.6344210000    0   0   0
Pt            2.7306234411        6.3061045231        9.3594310000    0   0   0
Pt            1.3653155429        8.6708839957       16.3472473898
Pt            2.7306221715        7.8826197992       13.9807332565
Pt            1.3653117203        7.0943682011       11.6344210000    0   0   0
Pt            1.3653117202        8.6708945770        9.3594310000    0   0   0
Pt            8.1918529878        1.5765365561       16.3472470691
Pt            9.5571618390        0.7882735064       13.9807363341
Pt            8.1918713045       -0.0000000006       11.6344210000    0   0   0
Pt            8.1918713044        1.5765263753        9.3594310000    0   0   0
Pt            6.8265457985        3.9413184184       16.3472476089
Pt            8.1918536386        3.1530577791       13.9807330558
Pt            6.8265595836        2.3647890733       11.6344210000    0   0   0
Pt            6.8265595835        3.9413154491        9.3594310000    0   0   0
Pt            5.4612382544        6.3060995578       16.3472497009
Pt            6.8265444294        5.5178407507       13.9807341494
Pt            5.4612478627        4.7295791271       11.6344210000    0   0   0
Pt            5.4612478626        6.3061045229        9.3594310000    0   0   0
Pt            4.0959311982        8.6708847198       16.3472515327
Pt            5.4612362969        7.8826227379       13.9807416081
Pt            4.0959361418        7.0943682009       11.6344210000    0   0   0
Pt            4.0959361417        8.6708945768        9.3594310000    0   0   0
 C                  3.95619779    5.17747681   18.32291712
 C                  2.95442915    6.17887277   18.34491198
 C                  1.74931835    5.51976820   18.42013420
 O                  1.93930433    4.17782698   18.45089274
 H                  5.03101126    5.30666171   18.24637459
 H                  3.09401738    7.25466563   18.30950534
 H                  0.71613894    5.85334029   18.44987249
 C                  3.75049106    2.58712572   18.41614957
 H                  2.92137736    1.83776279   18.44425772
 O                  4.92983530    2.23931121   18.40363741
 C                  3.28030354    4.06768486   18.39728890
--khouini fahime,PH.D student
 physical chemistry, university of zanjan
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