[Wannier] Issue with Wannierisation Step for Interface structure – Large Spread

Mainak Ghosh mainakg at iitb.ac.in
Thu May 1 18:36:59 CEST 2025



Hi all,

I am currently working on a system involving a Ni/SrTiO₃ (Ni/STO) 
interface and encountering persistent issues with the wannierise step in 
Wannier90.

System details:

     I am using norm-conserving LDA pseudopotentials.

     The DFT calculations were performed using Quantum ESPRESSO, and I 
have the SCF and NSCF files ready, along with the corresponding .win 
input file for Wannier90.

Here, is the _.win_ file,

  num_bands         =  200       # after looking at the nscf.out file
num_wann          =   78

!dis_froz_min      = -6.3
dis_froz_max      = 3.30  # after looking at the nscf.out file
dis_num_iter      =  500
dis_mix_ratio = 1.0

num_iter          = 30000     #gauge dependent term
conv_window=2        #gauge dependent term
conv_tol=1.0E-7      #gauge dependent term
#guiding_centres  =   true

spinors = T
begin projections
Ti:dxy;dyz;dxz
O:s;p
Ni:s;d
end projections

fermi_energy = 1.0770    # look  at the nscf.out file

restart = plot
bands_plot = true

# kpath = true
kpath_task = bands+curv
kpath_num_points=100
begin kpoint_path
G 0.0 0.0 0.0 X 0.5 0.0 0.0
X 0.5 0.0 0.0 M 0.5 0.5 0.0
M 0.5 0.5 0.0 G 0.0 0.0 0.0
end kpoint_path

# kslice = true
kslice_task = curv+fermi_lines
kslice_2dkmesh = 200 200
kslice_corner = -.5  -.5  0.0
kslice_b1 =     1.0 -0.0 -0.0
kslice_b2 =     0.0  1.0  0.0

#berry = true
#berry_task = ahc
#berry_kmesh = 360 360 60
#berry_curv_adpt_kmesh = 7
#berry_curv_adpt_kmesh_thresh = 100.0

begin unit_cell_cart
[ang]
3.9100000000         0.0000000000         0.0000000000
0.0000000000         3.9100000000         0.0000000000
0.0000000000         0.0000000000         20.000000000
end unit_cell_cart

begin atoms_cart
[ang]
Sr               0.0000000000        0.0000000000        2.1311168147
Ti               1.9550000430        1.9550000430        3.8931201239
O                1.9550000430        1.9550000430        1.8743186300
O                0.0000000000        1.9550000430        3.9186852638
O                1.9550000430        0.0000000000        3.9186852638
Ni               0.0000000000        0.0000000000        7.1677945000
Ni               1.9550000430        1.9550000430        7.2152896910
Ni               1.9550000430        0.0000000000        5.8504948569
Ni               0.0000000000        1.9550000430        5.8504948569
end atoms_cart

mp_grid           = 12 12 2

begin kpoints
   0.00000000  0.00000000  0.00000000  3.472222e-03
   0.00000000  0.00000000  0.50000000  3.472222e-03
   0.00000000  0.08333333  0.00000000  3.472222e-03
   0.00000000  0.08333333  0.50000000  3.472222e-03
   0.00000000  0.16666667  0.00000000  3.472222e-03
   0.00000000  0.16666667  0.50000000  3.472222e-03
   0.00000000  0.25000000  0.00000000  3.472222e-03
   0.00000000  0.25000000  0.50000000  3.472222e-03
   0.00000000  0.33333333  0.00000000  3.472222e-03
   0.00000000  0.33333333  0.50000000  3.472222e-03
   0.00000000  0.41666667  0.00000000  3.472222e-03
...................................................

Convergence behavior:

     The disentanglement threshold (conv_thr) reaches after 232 steps.

          228     105.01714841     105.01714839       1.180E-10    799.41 
    <-- DIS
      229     105.01714839     105.01714837       1.023E-10    802.92    
<-- DIS
      230     105.01714837     105.01714836       8.862E-11    806.42    
<-- DIS
      231     105.01714835     105.01714834       7.676E-11    809.93    
<-- DIS
      232     105.01714833     105.01714833       6.646E-11    813.43    
<-- DIS

              <<<      Delta < 1.000E-10  over  3 iterations     >>>
              <<< Disentanglement convergence criteria satisfied >>>

         Final Omega_I   105.01714833 (Ang^2)

  
+----------------------------------------------------------------------------+

PROBLEM

  But the total spread in wannierise step in Ni s orbital is very high 
and wannierise criterial is not satisfying even after 30000 steps,

      30000    -0.175E-01     6.2504642182      252.8300328556   31277.28 
  <-- CONV
         O_D=     11.1019693 O_OD=    136.7109152 O_TOT=    252.8300329 
<-- SPRD
  Delta: O_D=  0.2488336E-03 O_OD= -0.1775718E-01 O_TOT= -0.1750834E-01 
<-- DLTA
  
------------------------------------------------------------------------------

  Writing checkpoint file ni.chk... done

  Final State
   WF centre and spread    1  (  1.944998,  1.953929,  3.871577 )     
2.86732237
   WF centre and spread    2  (  1.966949,  1.954736,  3.868485 )     
2.57381341
   WF centre and spread    3  (  1.955545,  1.952317,  3.868975 )     
2.89108230
   WF centre and spread    4  (  1.955233,  1.960370,  3.854742 )     
2.65311230
   WF centre and spread    5  (  1.954614,  1.954374,  3.852336 )     
1.36214252
   WF centre and spread    6  (  1.955959,  1.955650,  3.853556 )     
1.30514171
   WF centre and spread    7  (  1.955050,  1.955183,  1.854926 )     
0.51999192
   WF centre and spread    8  (  1.955009,  1.954735,  1.855535 )     
0.51768366
   WF centre and spread    9  (  1.955749,  1.962201,  1.826277 )     
2.06833330
   WF centre and spread   10  (  1.955634,  1.945553,  1.777685 )     
2.31329943
   WF centre and spread   11  (  1.953439,  1.954892,  1.870298 )     
1.21739379
   WF centre and spread   12  (  1.957857,  1.954900,  1.869626 )     
1.19974782
   WF centre and spread   13  (  1.954958,  1.955417,  1.870230 )     
1.21822751
   WF centre and spread   14  (  1.955021,  1.954587,  1.868733 )     
1.20703135
   WF centre and spread   15  (  0.000050,  1.955050,  3.922437 )     
0.52667372
   WF centre and spread   16  ( -0.000124,  1.954870,  3.922757 )     
0.53334483
   WF centre and spread   17  ( -0.000059,  1.955449,  3.877855 )     
1.16077505
   WF centre and spread   18  (  0.000161,  1.954583,  3.865140 )     
1.24476743
   WF centre and spread   19  ( -0.000245,  1.954986,  3.918835 )     
1.04528812
   WF centre and spread   20  (  0.000569,  1.954980,  3.918970 )     
1.06294809
   WF centre and spread   21  ( -0.000052,  1.954436,  3.890782 )     
0.95967486
   WF centre and spread   22  (  0.000052,  1.956091,  3.885915 )     
0.97439535
   WF centre and spread   23  (  1.955034,  0.000030,  3.922569 )     
0.52664258
   WF centre and spread   24  (  1.954906, -0.000105,  3.922709 )     
0.53346347
   WF centre and spread   25  (  1.954965, -0.000151,  3.877452 )     
1.16270267
   WF centre and spread   26  (  1.955162,  0.000328,  3.867416 )     
1.23203641
   WF centre and spread   27  (  1.954116, -0.000052,  3.890908 )     
0.95776762
   WF centre and spread   28  (  1.956759,  0.000128,  3.887213 )     
0.96688369
   WF centre and spread   29  (  1.955025,  0.000293,  3.918855 )     
1.04582357
   WF centre and spread   30  (  1.954992, -0.000154,  3.918954 )     
1.06393295
   WF centre and spread   31  ( -0.026052,  0.056334,  3.977308 )    
32.95594719
   WF centre and spread   32  ( -0.030055,  0.136790,  3.996386 )    
34.48003072
   WF centre and spread   33  ( -0.000149, -0.000159,  7.188095 )     
0.66393628
   WF centre and spread   34  (  0.000353,  0.000435,  7.193201 )     
0.72185264
   WF centre and spread   35  (  0.000296,  0.000165,  7.143434 )     
0.70260985
   WF centre and spread   36  ( -0.000700, -0.000349,  7.133028 )     
0.78293750
   WF centre and spread   37  (  0.000198,  0.000041,  7.144084 )     
0.70487274
   WF centre and spread   38  ( -0.000850, -0.001949,  7.133512 )     
0.78372333
   WF centre and spread   39  ( -0.000501, -0.001541,  7.151121 )     
0.71308269
   WF centre and spread   40  (  0.000505,  0.001869,  7.147888 )     
0.82103565
   WF centre and spread   41  (  0.000645,  0.003330,  7.155581 )     
0.85948011
   WF centre and spread   42  (  0.000135, -0.001240,  7.152173 )     
0.97712655
   WF centre and spread   43  (  2.010446,  2.063570,  7.295221 )     
9.70842298
   WF centre and spread   44  (  1.897820,  1.898118,  7.248419 )     
9.98760740
   WF centre and spread   45  (  1.955007,  1.955429,  7.244020 )     
0.63777597
   WF centre and spread   46  (  1.955247,  1.955275,  7.244263 )     
0.68213596
   WF centre and spread   47  (  1.954026,  1.955272,  7.228405 )     
0.79656210
   WF centre and spread   48  (  1.955731,  1.954666,  7.227726 )     
0.89167342
   WF centre and spread   49  (  1.955147,  1.953315,  7.228365 )     
0.80009785
   WF centre and spread   50  (  1.954822,  1.956289,  7.227845 )     
0.89384518
   WF centre and spread   51  (  1.955453,  1.954730,  7.197972 )     
0.76949331
   WF centre and spread   52  (  1.954986,  1.954946,  7.194837 )     
0.90608407
   WF centre and spread   53  (  1.954870,  1.955008,  7.207880 )     
0.76393179
   WF centre and spread   54  (  1.956844,  1.958469,  7.205129 )     
0.85689564
   WF centre and spread   55  (  2.068709,  0.215411,  4.812913 )    
24.74338945
   WF centre and spread   56  (  1.921542, -0.291115,  5.353400 )    
22.44239477
   WF centre and spread   57  (  1.954953, -0.000363,  5.908412 )     
0.73422585
   WF centre and spread   58  (  1.955223, -0.000005,  5.906879 )     
0.82446194
   WF centre and spread   59  (  1.954829, -0.000281,  5.898759 )     
0.66155912
   WF centre and spread   60  (  1.954575,  0.000851,  5.904668 )     
0.70959046
   WF centre and spread   61  (  1.955062,  0.002286,  5.909930 )     
0.81494571
   WF centre and spread   62  (  1.954747,  0.001346,  5.911470 )     
0.87933931
   WF centre and spread   63  (  1.954888,  0.000276,  5.839626 )     
0.84709073
   WF centre and spread   64  (  1.956725,  0.002402,  5.830453 )     
1.05782795
   WF centre and spread   65  (  1.954993, -0.000101,  5.848045 )     
0.75000652
   WF centre and spread   66  (  1.952838, -0.001786,  5.846900 )     
0.82053137
   WF centre and spread   67  (  0.209518,  1.982586,  4.962810 )    
26.01437663
   WF centre and spread   68  ( -0.202086,  1.767255,  5.409431 )    
21.69650049
   WF centre and spread   69  ( -0.000082,  1.955077,  5.909168 )     
0.73315158
   WF centre and spread   70  (  0.000010,  1.955150,  5.905662 )     
0.82022039
   WF centre and spread   71  (  0.000634,  1.954979,  5.909152 )     
0.81139578
   WF centre and spread   72  (  0.000297,  1.954797,  5.913492 )     
0.88199384
   WF centre and spread   73  ( -0.000377,  1.953713,  5.898770 )     
0.66254059
   WF centre and spread   74  (  0.000534,  1.956269,  5.905731 )     
0.71070569
   WF centre and spread   75  (  0.000211,  1.955226,  5.839593 )     
0.84140507
   WF centre and spread   76  (  0.001551,  1.956912,  5.832332 )     
1.04576502
   WF centre and spread   77  (  0.000583,  1.955842,  5.848196 )     
0.74575013
   WF centre and spread   78  ( -0.000875,  1.953654,  5.847708 )     
0.80823159
   Sum of centres and spreads ( 89.970551, 89.948800,404.791137 )   
252.83000469

          Spreads (Ang^2)       Omega I      =   105.017148326
         ================       Omega D      =    11.101969314
                                Omega OD     =   136.710915215
     Final Spread (Ang^2)       Omega Total  =   252.830032856
  
------------------------------------------------------------------------------
  Time for wannierise        30379.377 (sec)

Any suggestions will be helpful for me.

I have attached the .scf and .nscf files in the following

Thanks in advance

Mainak Ghosh

Postdoc, Dept. of Physics

IIT Bombay, India
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