[QE-users] c_bands: eigenvalues not converged

Otani Minoru otani at ccs.tsukuba.ac.jp
Thu May 26 05:19:09 CEST 2022


Dear Tom,

A few days ago, we had almost the same question about the c_bands with ESM calculation. I understand that the diagonalization method affects the number of warning messages. Although it takes time to get a converged result, the "cg" method reduces the number of messages.

I also realized a different SCF convergence behavior in PBC and BC1, even in a neutral charge and unpolarized slab calculation. (Basically, those two calculations are identical. Thus, we can expect that the behavior is the same)
I will check more detail about this. I hope the cg method can be your workaround. I think the following posts will help you:
https://lists.quantum-espresso.org/pipermail/users/2018-May/040686.html
https://lists.quantum-espresso.org/pipermail/users/2020-July/045293.html

By the way, I usually use mixing_mode = ‘plain’.

Best regards,
Minoru
--------------------------------------------------------------------------------------------------------
Minoru Otani, Ph.D., Professor
Center for Computational Sciences and Faculty of Pure and Applied Sciences, 
University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki 305-8577, Japan
TEL: +81-29-853-4273
FAX: +81-29-853-6406
E-mail: otani at ccs.tsukuba.ac.jp
Web: https://www2.ccs.tsukuba.ac.jp/public/otani/
--------------------------------------------------------------------------------------------------------

> On May 25, 2022, at 21:23, Tom Demeyere <T.Demeyere at soton.ac.uk> wrote:
> 
> Dear users,
> 
> I recently changed pseudopotential for my Pt(111) slab calculations (I changed to the USPP one given by SSSP efficiency). I did a vc-relax to get the alat for this pseudopotential and built the surface using ASE. 
> 
> The calculation converges quite well (~ 30 steps) but at every step, I have the message:
> 
> c_bands:  X eigenvalues not converged
> 
> X is usually between 1 and 4, the warning also appears at the last step of the self-consistency. After the first geometry step, it still appears but less frequently. I don’t know if this is a really big issue but I would like to know why it happens.
> 
> Here is my input (I use ESM-BC1)
> 
> %%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%
> 
> &CONTROL
>  calculation = 'relax'
>  etot_conv_thr = 1.0000000000d-05, forc_conv_thr = 5.0000000000d-04
>  tprnfor = .true., tstress = .false.
>  verbosity = 'high'
> /
> &SYSTEM
>  ibrav = 0
>  ecutwfc = 60, ecutrho = 480
>  nat = 45, ntyp = 1
>  occupations = 'smearing', smearing = 'cold', degauss = 0.01
>  assume_isolated = "esm", esm_bc = "bc1"
> /
> &ELECTRONS
>  conv_thr = 1.00d-8
>  mixing_mode = "local-TF", mixing_beta = 0.4
> /
> &IONS
>  ion_dynamics = "bfgs"
> /
> ATOMIC_SPECIES
> Pt 195.084 pt_pbe_v1.4.uspp.F.UPF
> ATOMIC_POSITIONS angstrom
> Pt      -0.28031804       2.02302122      -4.57757447
> Pt       2.52286238       2.02302122      -4.57757447
> Pt       5.32604281       2.02302122      -4.57757447
> Pt       1.12127217       4.45064668      -4.57757447
> Pt       3.92445260       4.45064668      -4.57757447
> Pt       6.72763302       4.45064668      -4.57757447
> Pt       2.52286238       6.87827214      -4.57757447
> Pt       5.32604281       6.87827214      -4.57757447
> Pt       8.12922324       6.87827214      -4.57757447
> Pt      -0.28031804       0.40460424      -2.28878724
> Pt       2.52286238       0.40460424      -2.28878724
> Pt       5.32604281       0.40460424      -2.28878724
> Pt       1.12127217       2.83222970      -2.28878724
> Pt       3.92445260       2.83222970      -2.28878724
> Pt       6.72763302       2.83222970      -2.28878724
> Pt       2.52286238       5.25985516      -2.28878724
> Pt       5.32604281       5.25985516      -2.28878724
> Pt       8.12922324       5.25985516      -2.28878724
> Pt       1.12127217       1.21381273       0.00000000
> Pt       3.92445260       1.21381273       0.00000000
> Pt       6.72763302       1.21381273       0.00000000
> Pt       2.52286238       3.64143819       0.00000000
> Pt       5.32604281       3.64143819       0.00000000
> Pt       8.12922324       3.64143819       0.00000000
> Pt       3.92445260       6.06906365       0.00000000
> Pt       6.72763302       6.06906365       0.00000000
> Pt       9.53081345       6.06906365       0.00000000
> Pt      -0.28031804       2.02302122       2.28878723
> Pt       2.52286238       2.02302122       2.28878723
> Pt       5.32604281       2.02302122       2.28878723
> Pt       1.12127217       4.45064668       2.28878723
> Pt       3.92445260       4.45064668       2.28878723
> Pt       6.72763302       4.45064668       2.28878723
> Pt       2.52286238       6.87827214       2.28878723
> Pt       5.32604281       6.87827214       2.28878723
> Pt       8.12922324       6.87827214       2.28878723
> Pt      -0.28031804       0.40460424       4.57757447
> Pt       2.52286238       0.40460424       4.57757447
> Pt       5.32604281       0.40460424       4.57757447
> Pt       1.12127217       2.83222970       4.57757447
> Pt       3.92445260       2.83222970       4.57757447
> Pt       6.72763302       2.83222970       4.57757447
> Pt       2.52286238       5.25985516       4.57757447
> Pt       5.32604281       5.25985516       4.57757447
> Pt       8.12922324       5.25985516       4.57757447
> K_POINTS automatic
> 4 4 1 0 0 0
> CELL_PARAMETERS angstrom
> 8.409541279253872  0.000000000000000   0.000000000000000
> 4.204770639626936  7.282876382007739   0.000000000000000
> 0.000000000000000  0.000000000000000  40.000000000000000
> 
> %%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%
> 
> -----------------------------------------
> Tom Demeyere MSc
> PhD student
> Skylaris Research Group
> School of Chemistry, University of Southampton
> 
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