[QE-users] How to properly restart CI-NEB? convergence issues

Oskar Cheong oskarcheong at gmail.com
Sun Mar 14 20:47:55 CET 2021


Hello QE Team,
thank you for this nice forum here. I have an issue when restarting with
CI-NEB.
1. Usually I start out with NEB with "no-CI". Then after this calculation
converges, I restart my calculation with the same input script and switch
to "auto" and restart my CI-NEB. However, oftentimes convergence is not
reached.
I tried to follow the rules here with running "no-CI" then "auto". Can you
maybe tell me how to properly start my CI-NEB ("auto") when my previous NEB
calculation without CI has converged?


2. Also, I am not sure whether it is a bug or something, but when I
manually restart my calculation of NEB, I usually take the structure from
.crd file and copy and paste it in the input file. When I have only Final
and Last image, the simulation runs smoothly, but whenever I paste the
coordinates for intermediate images inside the input file, I get an error
message:

"xml_AddCharacter: Invalid character in chars"

[image: image.png]

I realised it only happens when I include intermediate images. Please find
my input file below.

BEGIN
BEGIN_PATH_INPUT
&PATH
  restart_mode      = 'from_scratch'
  string_method     = 'neb',
  nstep_path        = 1000,
  ds                = 1.D0,
  opt_scheme        = "broyden",
  num_of_images     = 5,
  CI_scheme         = "no-CI",
  path_thr          = 0.05D0,
/
END_PATH_INPUT
BEGIN_ENGINE_INPUT
&CONTROL
  prefix         = 'Pt'
  pseudo_dir      = './'
  outdir          = './'
  etot_conv_thr   = 1.0e-4
  forc_conv_thr   = 1.0e-3
  disk_io         = 'low'
  tstress         = .true.
  tprnfor           = .true.
  max_seconds     = 85000
/
&SYSTEM
    ibrav           = 0
    nat             = 50
    ntyp            = 3
    ecutwfc         = 50.0
    ecutrho         = 200.0
    input_DFT       = 'pbe'
    occupations     = 'smearing'
    smearing        = 'gaussian'
    degauss         = 0.02
    nosym           = .true.
/
&ELECTRONS
    diagonalization = 'david'
    electron_maxstep= 1000
    conv_thr        = 1.0e-6
    mixing_beta     = 0.3
/
&IONS
/
ATOMIC_SPECIES
Pt     195.084  Pt.pbe-n-kjpaw_psl.1.0.0.UPF
H     1.0    H.pbe-kjpaw_psl.1.0.0.UPF
C     12.01  C.pbe-n-kjpaw_psl.1.0.0.UPF
BEGIN_POSITIONS
FIRST_IMAGE
ATOMIC_POSITIONS (angstrom)
Pt      0.0000  0.0000  10.0000 0       0       0
Pt      5.6286  4.8745  10.0000 0       0       0
Pt      2.8143  0.0000  10.0000 0       0       0
Pt      5.6286  0.0000  10.0000 0       0       0
Pt      4.2214  2.4372  10.0000 0       0       0
Pt      7.0357  2.4372  10.0000 0       0       0
Pt      2.8143  4.8745  10.0000 0       0       0
Pt      1.4071  2.4372  10.0000 0       0       0
Pt      8.4429  4.8745  10.0000 0       0       0
Pt      9.8500  4.0621  12.2979 0       0       0
Pt      5.6286  6.4993  12.2979 0       0       0
Pt      8.4429  1.6248  12.2979 0       0       0
Pt      11.2571 6.4993  12.2979 0       0       0
Pt      5.6286  1.6248  12.2979 0       0       0
Pt      8.4429  6.4993  12.2979 0       0       0
Pt      2.8143  1.6248  12.2979 0       0       0
Pt      4.2214  4.0621  12.2979 0       0       0
Pt      7.0357  4.0621  12.2979 0       0       0
Pt      8.4424  3.2667  14.5822
Pt      7.0409  0.8263  14.5649
Pt      9.8552  5.7001  14.5651
Pt      7.0411  5.6948  14.5830
Pt      5.6399  3.2666  14.5824
Pt      1.4165  0.8282  14.5828
Pt      4.2229  0.8285  14.5835
Pt      2.8202  3.2588  14.5832
Pt      4.2271  5.7002  14.5650
Pt      7.0467  2.4820  16.8783
Pt      2.8256  0.0388  16.8723
Pt      9.8689  2.4600  16.8700
Pt      4.2233  2.4598  16.8727
Pt      11.2686 4.9020  16.8360
Pt      8.4525  0.0273  16.8355
Pt      8.4391  4.8946  16.8781
Pt      5.6404  0.0271  16.8358
Pt      5.6542  4.8941  16.8779
Pt      5.6349  6.5377  19.1512
Pt      8.4521  1.6570  19.1532
Pt      4.2344  4.1074  19.1533
Pt      8.4664  6.5378  19.1528
Pt      9.8694  4.1084  19.1508
Pt      2.8266  1.6633  19.2737
Pt      5.6474  1.6560  19.1529
Pt      7.0514  4.1010  19.3651
Pt      11.2724 6.5376  19.1503
C       7.0593  4.1235  21.4390
H       6.6870  3.1544  21.7906
H       6.4055  4.9377  21.7729
H       8.0899  4.2906  21.7738
H       2.8009  1.6863  20.8320
INTERMEDIATE_IMAGE
ATOMIC_POSITIONS (angstrom)
Pt      0.0000  0.0000  10.0000 0       0       0
Pt      5.6286  4.8745  10.0000 0       0       0
Pt      2.8143  0.0000  10.0000 0       0       0
Pt      5.6286  0.0000  10.0000 0       0       0
Pt      4.2214  2.4372  10.0000 0       0       0
Pt      7.0357  2.4372  10.0000 0       0       0
Pt      2.8143  4.8745  10.0000 0       0       0
Pt      1.4071  2.4372  10.0000 0       0       0
Pt      8.4429  4.8745  10.0000 0       0       0
Pt      9.8500  4.0621  12.2979 0       0       0
Pt      5.6286  6.4993  12.2979 0       0       0
Pt      8.4429  1.6248  12.2979 0       0       0
Pt      11.2571 6.4993  12.2979 0       0       0
Pt      5.6286  1.6248  12.2979 0       0       0
Pt      8.4429  6.4993  12.2979 0       0       0
Pt      2.8143  1.6248  12.2979 0       0       0
Pt      4.2214  4.0621  12.2979 0       0       0
Pt      7.0357  4.0621  12.2979 0       0       0
Pt      8.4141  3.2483  14.5861
Pt      7.0133  0.8085  14.5661
Pt      9.8251  5.6857  14.5588
Pt      7.0148  5.6788  14.5815
Pt      5.6076  3.2535  14.5982
Pt      1.3842  0.8086  14.5708
Pt      4.1985  0.8056  14.5643
Pt      2.7930  3.2473  14.5781
Pt      4.1987  5.6808  14.5769
Pt      6.9773  2.4386  16.8820
Pt      2.7560  -0.0205 16.8413
Pt      9.7939  2.4225  16.8466
Pt      4.1652  2.4279  16.8563
Pt      11.2060 4.8590  16.8503
Pt      8.3853  -0.0149 16.8380
Pt      8.3659  4.8515  16.8725
Pt      5.5726  -0.0186 16.8319
Pt      5.5641  4.8410  16.9151
Pt      5.5255  6.4711  19.1482
Pt      8.3481  1.5834  19.1454
Pt      4.0918  4.0054  19.2558
Pt      8.3500  6.4687  19.1465
Pt      9.7381  4.0371  19.1386
Pt      2.7095  1.5688  19.1462
Pt      5.5319  1.5725  19.1376
Pt      6.9307  4.0270  19.3367
Pt      11.1608 6.4682  19.1422
C       6.8583  3.9836  21.4053
H       6.5185  2.9866  21.7101
H       6.1451  4.7483  21.7328
H       7.8653  4.1902  21.7836
H       3.6773  3.6911  20.7378
INTERMEDIATE_IMAGE
ATOMIC_POSITIONS (angstrom)
Pt      0.0000  0.0000  10.0000 0       0       0
Pt      5.6286  4.8745  10.0000 0       0       0
Pt      2.8143  0.0000  10.0000 0       0       0
Pt      5.6286  0.0000  10.0000 0       0       0
Pt      4.2214  2.4372  10.0000 0       0       0
Pt      7.0357  2.4372  10.0000 0       0       0
Pt      2.8143  4.8745  10.0000 0       0       0
Pt      1.4071  2.4372  10.0000 0       0       0
Pt      8.4429  4.8745  10.0000 0       0       0
Pt      9.8500  4.0621  12.2979 0       0       0
Pt      5.6286  6.4993  12.2979 0       0       0
Pt      8.4429  1.6248  12.2979 0       0       0
Pt      11.2571 6.4993  12.2979 0       0       0
Pt      5.6286  1.6248  12.2979 0       0       0
Pt      8.4429  6.4993  12.2979 0       0       0
Pt      2.8143  1.6248  12.2979 0       0       0
Pt      4.2214  4.0621  12.2979 0       0       0
Pt      7.0357  4.0621  12.2979 0       0       0
Pt      8.4102  3.2602  14.6085
Pt      7.0106  0.8187  14.5759
Pt      9.8225  5.6907  14.5789
Pt      7.0109  5.6872  14.6128
Pt      5.6064  3.2578  14.6093
Pt      1.3842  0.8170  14.5906
Pt      4.1992  0.8165  14.5753
Pt      2.7894  3.2548  14.5904
Pt      4.1955  5.6933  14.5844
Pt      6.9707  2.4663  16.9214
Pt      2.7473  0.0084  16.8889
Pt      9.7841  2.4485  16.8785
Pt      4.1589  2.4561  16.8841
Pt      11.1926 4.8823  16.8725
Pt      8.3829  0.0066  16.8737
Pt      8.3528  4.8704  16.9403
Pt      5.5612  0.0067  16.8507
Pt      5.5777  4.8796  16.9353
Pt      5.5502  6.5265  19.2549
Pt      8.3390  1.6382  19.1927
Pt      4.1071  4.0748  19.2476
Pt      8.3399  6.5025  19.1953
Pt      9.7346  4.0696  19.2030
Pt      2.7113  1.6442  19.1905
Pt      5.5200  1.6151  19.1754
Pt      6.9054  4.0190  19.5666
Pt      11.1242 6.5227  19.1640
C       6.5607  3.7858  21.6460
H       6.2171  2.7608  21.8439
H       5.8173  4.4829  22.0581
H       7.5293  3.9692  22.1189
H       4.8384  5.3756  20.3119
INTERMEDIATE_IMAGE
ATOMIC_POSITIONS (angstrom)
Pt      0.0000  0.0000  10.0000 0       0       0
Pt      5.6286  4.8745  10.0000 0       0       0
Pt      2.8143  0.0000  10.0000 0       0       0
Pt      5.6286  0.0000  10.0000 0       0       0
Pt      4.2214  2.4372  10.0000 0       0       0
Pt      7.0357  2.4372  10.0000 0       0       0
Pt      2.8143  4.8745  10.0000 0       0       0
Pt      1.4071  2.4372  10.0000 0       0       0
Pt      8.4429  4.8745  10.0000 0       0       0
Pt      9.8500  4.0621  12.2979 0       0       0
Pt      5.6286  6.4993  12.2979 0       0       0
Pt      8.4429  1.6248  12.2979 0       0       0
Pt      11.2571 6.4993  12.2979 0       0       0
Pt      5.6286  1.6248  12.2979 0       0       0
Pt      8.4429  6.4993  12.2979 0       0       0
Pt      2.8143  1.6248  12.2979 0       0       0
Pt      4.2214  4.0621  12.2979 0       0       0
Pt      7.0357  4.0621  12.2979 0       0       0
Pt      8.4305  3.2508  14.5722
Pt      7.0230  0.8148  14.5726
Pt      9.8366  5.6879  14.5742
Pt      7.0227  5.6893  14.5706
Pt      5.6151  3.2512  14.5706
Pt      1.3944  0.8146  14.5741
Pt      4.2078  0.8144  14.5730
Pt      2.8009  3.2509  14.5733
Pt      4.2078  5.6892  14.5707
Pt      7.0068  2.4400  16.8435
Pt      2.7869  0.0036  16.8479
Pt      9.8213  2.4413  16.8508
Pt      4.1928  2.4402  16.8458
Pt      11.2279 4.8799  16.8461
Pt      8.4120  0.0034  16.8465
Pt      8.4151  4.8796  16.8450
Pt      5.6003  0.0026  16.8462
Pt      5.5990  4.8798  16.8401
Pt      5.5828  6.5149  19.1386
Pt      8.3984  1.6290  19.1485
Pt      4.1672  4.0682  19.1352
Pt      8.3990  6.5087  19.1505
Pt      9.8071  4.0690  19.1506
Pt      2.7688  1.6308  19.1515
Pt      5.5826  1.6261  19.1406
Pt      7.0016  4.0676  19.1287
Pt      11.2110 6.5069  19.1534
C       5.9976  3.9723  22.2288
H       5.8501  2.8885  22.2957
H       5.7225  4.4577  23.1708
H       7.0530  4.1843  22.0080
H       5.3524  4.3885  21.4312
LAST_IMAGE
ATOMIC_POSITIONS (angstrom)
Pt      0.0000  0.0000  10.0000 0       0       0
Pt      5.6286  4.8745  10.0000 0       0       0
Pt      2.8143  0.0000  10.0000 0       0       0
Pt      5.6286  0.0000  10.0000 0       0       0
Pt      4.2214  2.4372  10.0000 0       0       0
Pt      7.0357  2.4372  10.0000 0       0       0
Pt      2.8143  4.8745  10.0000 0       0       0
Pt      1.4071  2.4372  10.0000 0       0       0
Pt      8.4429  4.8745  10.0000 0       0       0
Pt      9.8500  4.0621  12.2979 0       0       0
Pt      5.6286  6.4993  12.2979 0       0       0
Pt      8.4429  1.6248  12.2979 0       0       0
Pt      11.2571 6.4993  12.2979 0       0       0
Pt      5.6286  1.6248  12.2979 0       0       0
Pt      8.4429  6.4993  12.2979 0       0       0
Pt      2.8143  1.6248  12.2979 0       0       0
Pt      4.2214  4.0621  12.2979 0       0       0
Pt      7.0357  4.0621  12.2979 0       0       0
Pt      8.4390  3.2543  14.5731
Pt      7.0340  0.8180  14.5743
Pt      9.8480  5.6929  14.5760
Pt      7.0318  5.6924  14.5729
Pt      5.6258  3.2563  14.5732
Pt      1.4047  0.8174  14.5738
Pt      4.2180  0.8184  14.5750
Pt      2.8131  3.2544  14.5737
Pt      4.2201  5.6924  14.5733
Pt      7.0293  2.4476  16.8501
Pt      2.8088  0.0096  16.8500
Pt      9.8450  2.4476  16.8501
Pt      4.2177  2.4477  16.8515
Pt      11.2526 4.8845  16.8496
Pt      8.4380  0.0097  16.8503
Pt      8.4375  4.8843  16.8482
Pt      5.6236  0.0107  16.8517
Pt      5.6234  4.8842  16.8531
Pt      5.6212  6.5127  19.1603
Pt      8.4346  1.6377  19.1600
Pt      4.2147  4.0756  19.1648
Pt      8.4353  6.5124  19.1601
Pt      9.8424  4.0765  19.1600
Pt      2.8077  1.6374  19.1611
Pt      5.6214  1.6401  19.1611
Pt      7.0275  4.0754  19.1641
Pt      11.2500 6.5125  19.1618
C       5.5680  4.0330  23.0743
H       5.1554  3.0796  22.7232
H       5.4764  4.0926  24.1657
H       6.6254  4.1001  22.7906
H       5.0131  4.8607  22.6148
END_POSITIONS

CELL_PARAMETERS angstrom
8.44285496736738 0.00000000000000 0.00000000000000
4.22142748368369 7.31172688220779 0.00000000000000
0.00000000000000 0.00000000000000 29.19141628549884

K_POINTS (automatic)
 4 4 1 0 0 0
END_ENGINE_INPUT
END




Thank you for your help.


Kind regards,

Oskar
-------------- next part --------------
An HTML attachment was scrubbed...
URL: <http://lists.quantum-espresso.org/pipermail/users/attachments/20210314/ea9e2962/attachment.html>
-------------- next part --------------
A non-text attachment was scrubbed...
Name: image.png
Type: image/png
Size: 31415 bytes
Desc: not available
URL: <http://lists.quantum-espresso.org/pipermail/users/attachments/20210314/ea9e2962/attachment.png>


More information about the users mailing list