[QE-users] Too many bands are not converged

Reem Abdel-Kader Ibrahim rai11 at fayoum.edu.eg
Mon Feb 8 22:48:58 CET 2021


Dear users,
I am working on doping graphene nanomesh with scandium. I did scf
calculation and it did well. Then I ran nscf, but always got an error
message: "*Too many bands are not converged*". I have tried to increase
*ecutwfc* from 45 to 80 , but got the same error. Also, I have tried to
decrease *conv_thr* to 1.0e-9, but the same error. However, I was working
with the graphene nanomesh without Sc atom, and the scf and nscf
calculations were doing well.

The input files are following:
scf.in:
&CONTROL
                 calculation = 'scf' ,
                 restart_mode = 'from_scratch' ,
                 pseudo_dir = '/psudo' ,
                 outdir = '/tmp',
                 prefix= 'gn.sc',
                 tstress = .true. ,
                 tprnfor = .true. ,
              forc_conv_thr = 1.00e-03,
        wf_collect=.true.,
        nstep = 200,
        max_seconds = 65000 ,

      verbosity = 'high' ,

/
&SYSTEM
                       ibrav = 0,
                   celldm(1) = 27.89615,
                         nat = 72,
                        ntyp = 3,
                        nspin=2,
                     starting_magnetization(1)= 0.5,

                     ecutwfc = 60.0 ,
                     ecutrho = 600.0 ,
                        nbnd = 280,
                 occupations = 'smearing' ,
                     degauss = 0.002 ,
                    smearing = 'fermi-dirac' ,
/
&ELECTRONS
                    conv_thr = 1.0e-8 ,
                 mixing_mode = 'local-TF' ,
                 mixing_beta = 0.2 ,
             diagonalization = 'david' ,

/
&IONS
     ion_dynamics      = 'damp',
     pot_extrapolation = 'second_order',
     wfc_extrapolation = 'second_order',

/
CELL_PARAMETERS
     0.8660254037844386   -0.5      0.000000000
     0.8660254037844386    0.5      0.000000000
     0.000000000     0.000000000    1.05

ATOMIC_SPECIES
  Sc     44.955912   Sc.pbe-spn-rrkjus_psl.1.0.0.UPF
  C     12.01070     C.pbe-n-rrkjus_psl.1.0.0.UPF
  H   1.00794        H.pbe-rrkjus_psl.1.0.0.UPF

ATOMIC_POSITIONS (angstrom)
Sc       0.075617968   0.289821895   0.000000000
C        1.841864350  -0.074257015   0.000000000
C        2.250599961  -1.349110971   0.000000000
C        2.237722708   1.230253072   0.000000000
C        3.644501279  -1.310104833   0.000000000
C        3.654938628   1.234205490   0.000000000
C        4.292823115  -2.522125909   0.000000000
C        4.298370551  -0.036748469   0.000000000
C        4.352481848   2.435357814   0.000000000
C        5.666428775  -2.501473702   0.000000000
C        5.678351741  -0.026836419   0.000000000
C        5.744806594   2.446140468   0.000000000
C        6.284959790  -3.754026165   0.000000000
C        6.337305147  -1.264814968   0.000000000
C        6.373876062   1.200778014   0.000000000
C        6.444521895   3.681593179   0.000000000
C        7.641960373  -3.764685380   0.000000000
C        7.705064112  -1.376983277   0.000000000
C        7.743671548   1.302833282   0.000000000
C        7.842694656   3.716345229   0.000000000
C        8.399892462  -4.905935272   0.000000000
C        8.259090301  -2.562973836   0.000000000
C        8.418611467   2.442431045   0.000000000
C        8.502099913   4.963849208   0.000000000
C        9.787113573  -4.746312031   0.000000000
C        9.900308327   5.039375902   0.000000000
C       10.504273974  -5.938831678   0.000000000
C       10.626663250  -3.602955133   0.000000000
C       10.639641789   3.891306250   0.000000000
C       10.653815005   6.207682579   0.000000000
C       11.807843603  -5.601366538   0.000000000
C       12.026935106   5.950104801   0.000000000
C       11.974061635  -3.492126259   0.000000000
C       11.955901485   3.683070230   0.000000000
C       12.776605263  -4.653156326   0.000000000
C       12.791049186   4.804715812   0.000000000
C       14.253877780  -4.929524766   0.000000000
C       14.439416299  -2.565560929   0.000000000
C       14.352077852   2.473824980   0.000000000
C       14.247549453   4.868093756   0.000000000
C       15.051611979  -3.787191507   0.000000000
C       14.980878190   3.693850665   0.000000000
C       15.063066205  -1.404019808   0.000000000
C       14.957437538   1.296267303   0.000000000
C       16.443735927  -3.737300312   0.000000000
C       16.436049694  -1.289010591   0.000000000
C       16.346270483   1.168826636   0.000000000
C       16.371457768   3.645270147   0.000000000
C       17.126378915  -2.504168042   0.000000000
C       17.081809145  -0.041251226   0.000000000
C       17.022902888   2.396219081   0.000000000
C       18.530591563  -2.476222874   0.000000000
C       18.419565958   2.392848872   0.000000000
C       18.473973168  -0.026645424   0.000000000
C       19.193815533  -1.239724815   0.000000000
C       19.157362299   1.203025712   0.000000000
C       20.603612002  -1.210523499   0.000000000
C       20.570744041   1.229762388   0.000000000
C       21.324504163   0.026242481   0.000000000
C       22.724016305   0.100687092   0.000000000
H       12.169490038  -2.430178108   0.000000000
H       13.414233784  -2.458009102   0.000000000
H       13.317389513   2.376349652   0.000000000
H        9.271593348  -2.478217927   0.000000000
H       14.368433407  -0.627056947   0.000000000
H       14.197939450   0.566359179   0.000000000
H       10.401649916  -2.568600783   0.000000000
H        8.467678881  -0.659843339   0.000000000
H        8.437925451   0.526289432   0.000000000
H        9.420142990   2.103789638   0.000000000
H       10.160696653   2.984838860   0.000000000
H       12.093674315   2.619954299   0.000000000
K_POINTS automatic
  12  12  1   0 0  0

nscf.in
&CONTROL
                 calculation = 'nscf' ,
                 restart_mode = 'from_scratch' ,
                 pseudo_dir = '/psudo' ,
                 outdir = '/tmp',
                 prefix= 'gn.sc',
                 tstress = .true. ,
                 tprnfor = .true. ,
              forc_conv_thr = 1.00e-03,
        wf_collect=.true.,
        nstep = 200,
        max_seconds = 65000 ,
        disk_io = 'high' ,
      verbosity = 'high' ,

/
&SYSTEM
                       ibrav = 0,
                   celldm(1) = 27.89615,
                         nat = 72,
                        ntyp = 3,
                        nspin=2,
                     starting_magnetization(1)= 0.5,

                     ecutwfc = 60.0 ,
                     ecutrho = 600.0 ,
                        nbnd = 300,
                 occupations = 'tetrahedra' ,


/
&ELECTRONS
                    conv_thr = 1.0e-8 ,
                 mixing_mode = 'local-TF' ,
                 mixing_beta = 0.2 ,
             diagonalization = 'cg' ,

/
&IONS
     ion_dynamics      = 'damp',
     pot_extrapolation = 'second_order',
     wfc_extrapolation = 'second_order',

/
CELL_PARAMETERS
     0.8660254037844386   -0.5      0.000000000
     0.8660254037844386    0.5      0.000000000
     0.000000000     0.000000000    1.05

ATOMIC_SPECIES
  Sc     44.955912   Sc.pbe-spn-rrkjus_psl.1.0.0.UPF
  C     12.01070     C.pbe-n-rrkjus_psl.1.0.0.UPF
  H   1.00794        H.pbe-rrkjus_psl.1.0.0.UPF

ATOMIC_POSITIONS (angstrom)
Sc       0.075617968   0.289821895   0.000000000
C        1.841864350  -0.074257015   0.000000000
C        2.250599961  -1.349110971   0.000000000
C        2.237722708   1.230253072   0.000000000
C        3.644501279  -1.310104833   0.000000000
C        3.654938628   1.234205490   0.000000000
C        4.292823115  -2.522125909   0.000000000
C        4.298370551  -0.036748469   0.000000000
C        4.352481848   2.435357814   0.000000000
C        5.666428775  -2.501473702   0.000000000
C        5.678351741  -0.026836419   0.000000000
C        5.744806594   2.446140468   0.000000000
C        6.284959790  -3.754026165   0.000000000
C        6.337305147  -1.264814968   0.000000000
C        6.373876062   1.200778014   0.000000000
C        6.444521895   3.681593179   0.000000000
C        7.641960373  -3.764685380   0.000000000
C        7.705064112  -1.376983277   0.000000000
C        7.743671548   1.302833282   0.000000000
C        7.842694656   3.716345229   0.000000000
C        8.399892462  -4.905935272   0.000000000
C        8.259090301  -2.562973836   0.000000000
C        8.418611467   2.442431045   0.000000000
C        8.502099913   4.963849208   0.000000000
C        9.787113573  -4.746312031   0.000000000
C        9.900308327   5.039375902   0.000000000
C       10.504273974  -5.938831678   0.000000000
C       10.626663250  -3.602955133   0.000000000
C       10.639641789   3.891306250   0.000000000
C       10.653815005   6.207682579   0.000000000
C       11.807843603  -5.601366538   0.000000000
C       12.026935106   5.950104801   0.000000000
C       11.974061635  -3.492126259   0.000000000
C       11.955901485   3.683070230   0.000000000
C       12.776605263  -4.653156326   0.000000000
C       12.791049186   4.804715812   0.000000000
C       14.253877780  -4.929524766   0.000000000
C       14.439416299  -2.565560929   0.000000000
C       14.352077852   2.473824980   0.000000000
C       14.247549453   4.868093756   0.000000000
C       15.051611979  -3.787191507   0.000000000
C       14.980878190   3.693850665   0.000000000
C       15.063066205  -1.404019808   0.000000000
C       14.957437538   1.296267303   0.000000000
C       16.443735927  -3.737300312   0.000000000
C       16.436049694  -1.289010591   0.000000000
C       16.346270483   1.168826636   0.000000000
C       16.371457768   3.645270147   0.000000000
C       17.126378915  -2.504168042   0.000000000
C       17.081809145  -0.041251226   0.000000000
C       17.022902888   2.396219081   0.000000000
C       18.530591563  -2.476222874   0.000000000
C       18.419565958   2.392848872   0.000000000
C       18.473973168  -0.026645424   0.000000000
C       19.193815533  -1.239724815   0.000000000
C       19.157362299   1.203025712   0.000000000
C       20.603612002  -1.210523499   0.000000000
C       20.570744041   1.229762388   0.000000000
C       21.324504163   0.026242481   0.000000000
C       22.724016305   0.100687092   0.000000000
H       12.169490038  -2.430178108   0.000000000
H       13.414233784  -2.458009102   0.000000000
H       13.317389513   2.376349652   0.000000000
H        9.271593348  -2.478217927   0.000000000
H       14.368433407  -0.627056947   0.000000000
H       14.197939450   0.566359179   0.000000000
H       10.401649916  -2.568600783   0.000000000
H        8.467678881  -0.659843339   0.000000000
H        8.437925451   0.526289432   0.000000000
H        9.420142990   2.103789638   0.000000000
H       10.160696653   2.984838860   0.000000000
H       12.093674315   2.619954299   0.000000000
K_POINTS automatic
  24  24  1   0 0  0

,can anyone help me with this issue?

Regards,
Reem
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