[QE-users] Does order of atoms matter in Quantum Espresso?

Sheikh Ziauddin Ahmed sza9wz at virginia.edu
Mon Jan 6 02:26:21 CET 2020


Thanks. I am trying to calculate the phonon dispersion of a superlattice
consisting of InAs and AlSb. However, I am ending up with negative phonon
frequencies for the structure. I used the epsil flag. But that did not
help. How I can eliminate the negative phonon modes?

For relaxation I am using the following input:
&control
    calculation='vc-relax'
    restart_mode='from_scratch',
    prefix='AlInAsSb'
    tstress = .true. ,
    tprnfor = .true. ,
    verbosity ='high'
    etot_conv_thr=1.0D-12
    forc_conv_thr=1.0D-7
 /
 &system
    ibrav=0, nat=10, ntyp=4,
    ecutwfc = 50, ecutrho = 500
 /
 &electrons
    electron_maxstep=1000
    conv_thr    = 1.0e-9
    mixing_beta = 0.7
    mixing_mode = 'local-TF'
 /
 /
&IONS
/
&CELL
 cell_dofree = 'z'
/
ATOMIC_SPECIES
 Sb 121.76   Sb.pz-n-rrkjus_psl.1.0.0.UPF
 Al 26.98  Al.pz-n-rrkjus_psl.0.1.UPF
 As 74.92      As.pz-n-rrkjus_psl.0.2.UPF
 In 114.82     In.pz-dn-rrkjus_psl.0.2.2.UPF
ATOMIC_POSITIONS {angstrom}
Sb 0.00000000  0.00000000  0.00000000
Sb 0.00000000  3.04570000  3.07106916
Sb 0.00000000  0.00000000  6.14213831
Al 1.52285000  1.52285000  1.53553458
Al -1.52285000  1.52285000  4.60660373
Al 1.52285000  1.52285000  7.67767289
As 0.00000000  3.04570000  9.21320747
As 0.00000000  0.00000000  12.24743004
In -1.52285000  1.52285000  10.73031875
In 1.52285000  1.52285000  13.76454133
K_POINTS automatic
6 6 6 0 0 0
CELL_PARAMETERS {angstrom}
3.0457000000   3.0457000000   0.0000000000
-3.0457000000   3.0457000000   0.0000000000
0.0000000000   0.0000000000   15.2816526121


For SCF run:
&control
    calculation='scf'
    restart_mode='from_scratch',
    tstress = .true. ,
    tprnfor = .true. ,
 /
 &system
    ibrav=0, nat=10, ntyp=4,
    ecutwfc = 50, ecutrho = 500
 /
 &electrons
    conv_thr    = 1.0e-9
    mixing_beta = 0.7
    mixing_mode = 'local-TF'
 /
ATOMIC_SPECIES
  Sb 121.76   Sb.pz-n-rrkjus_psl.1.0.0.UPF
 Al 26.98  Al.pz-n-rrkjus_psl.0.1.UPF
 As 74.92      As.pz-n-rrkjus_psl.0.2.UPF
 In 114.82     In.pz-dn-rrkjus_psl.0.2.2.UPF
ATOMIC_POSITIONS {angstrom}
Sb       0.000000000   0.000000000   0.280559797
Sb       0.000000000   3.045700000   3.229150822
Sb       0.000000000   0.000000000   6.101422626
Al       1.522850000   1.522850000   1.784998522
Al      -1.522850000   1.522850000   4.668823707
Al       1.522850000   1.522850000   7.525405573
As       0.000000000   3.045700000   8.683670011
As       0.000000000   0.000000000  11.527025485
In      -1.522850000   1.522850000  10.092147868
In       1.522850000   1.522850000  13.117431792
K_POINTS automatic
6 6 6 0 0 0
CELL_PARAMETERS {angstrom}
   3.045700000   3.045700000   0.000000000
  -3.045700000   3.045700000   0.000000000
   0.000000000   0.000000000  14.843532218


On Thu, Jan 2, 2020 at 3:54 PM Paolo Giannozzi <p.giannozzi at gmail.com>
wrote:

> On Mon, Dec 30, 2019 at 11:08 PM Sheikh Ziauddin Ahmed <
> sza9wz at virginia.edu> wrote:
>
> I am trying to calculate the phonon dispersion of AlSb. I am getting two
>> different results depending on how I am introducing the atoms in the SCF
>> calculation. Will the order of the atom change the symmetry of the zinc
>> blende AlSb?
>>
>
> no. See attached.
>
> PG
>
>
>> In the first case the input deck is:
>> &system
>>     ibrav=2, nat=2, ntyp=2,
>>     ecutwfc = 50, ecutrho = 500,
>>     occupations='smearing',
>>     smearing='gauss',
>>     degauss=0.05,
>>     celldm(1)=11.5944146,
>>  /
>>  &electrons
>>     conv_thr    = 1.0e-12
>>     mixing_beta = 0.7
>>     mixing_mode = 'local-TF'
>>  /
>> ATOMIC_SPECIES
>>  Al 26.98 al_lda_v1.uspp.F.UPF
>>  Sb 121.76 sb_lda_v1.4.uspp.F.UPF
>> ATOMIC_POSITIONS (alat)
>>  Al 0.0   0.0   0.0
>>  Sb 0.25  0.25  0.25
>> K_POINTS automatic
>> 6 6 6 0 0 0
>>
>> In the second case the input deck is:
>>  &system
>>     ibrav=2, nat=2, ntyp=2,
>>     ecutwfc = 50, ecutrho = 500,
>>     !occupations='smearing',
>>     !smearing='gauss',
>>     !degauss=0.05,
>>     celldm(1)=11.5944146,
>>  /
>>  &electrons
>>     conv_thr    = 1.0e-12
>>     mixing_beta = 0.7
>>     mixing_mode = 'local-TF'
>>  /
>> ATOMIC_SPECIES
>>  Sb 121.76 sb_lda_v1.4.uspp.F.UPF
>>  Al 26.98 al_lda_v1.uspp.F.UPF
>> ATOMIC_POSITIONS (alat)
>>  Sb 0.0   0.0   0.0
>>  Al 0.25  0.25  0.25
>> K_POINTS automatic
>> 6 6 6 0 0 0
>>
>> Thanks in advance!
>> --
>> *Sheikh Ziauddin Ahmed *
>> PhD Candidate
>> Charles L. Brown Department of Electrical and Computer Engineering
>> University of Virginia
>> Email:sza9wz*@virginia.edu* <sza9wz at virginia.edu>
>> LinkedIn: https://www.linkedin.com/in/sheikh-ziauddin-ahmed
>> _______________________________________________
>> Quantum ESPRESSO is supported by MaX (www.max-centre.eu/quantum-espresso)
>> users mailing list users at lists.quantum-espresso.org
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>
>
>
> --
> Paolo Giannozzi, Dip. Scienze Matematiche Informatiche e Fisiche,
> Univ. Udine, via delle Scienze 208, 33100 Udine, Italy
> Phone +39-0432-558216, fax +39-0432-558222
>
>

-- 
*Sheikh Ziauddin Ahmed *
PhD Candidate
Charles L. Brown Department of Electrical and Computer Engineering
University of Virginia
Email:sza9wz*@virginia.edu* <sza9wz at virginia.edu>
LinkedIn: https://www.linkedin.com/in/sheikh-ziauddin-ahmed
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