[Pw_forum] How to select unit cell for optimization calculation?

Giovanni Cantele giovanni.cantele at spin.cnr.it
Tue Jul 7 10:01:56 CEST 2015


As far as I understand, the LiMn2O4 has 8 formula units in one unit cell, so you definitely need 56 atoms in the unit cell.

The cif file contains only information on the inequivalent atoms, all others can be obtained from the former by applying the
coordinate transformation of the space group Fd-3m

A useful way to do that, as specified here:

http://www.quantum-espresso.org/faq/input-data/#3.2 <http://www.quantum-espresso.org/faq/input-data/#3.2>

is to run the converter from cif files included in the QE distribution.

			espresso-5.2.0/PW/tools/cif2qe.sh 1513984 > 1513984.scf.in

This produces a file (that you might want to check for correctness and to modify according to your needs) that looks like


&CONTROL
                       title = '1513984'
                 calculation = 'relax'
                restart_mode = 'from_scratch'
                      outdir = './1'
                  pseudo_dir = '../PP/atompaw'
                      prefix = '1513984'
                     disk_io = 'none'
                   verbosity = 'default'
               etot_conv_thr = 0.0001
               forc_conv_thr = 0.001
                       nstep = 400
                     tstress = .true.
                     tprnfor = .true.
 /
 &SYSTEM
                       ibrav = 0
                         nat = 56
                        ntyp = 3
                     ecutwfc = 60
                     ecutrho = 480
                    vdw_corr = 'xdm'
                      xdm_a1 = 1.2153
                      xdm_a2 = 2.3704
 /
 &ELECTRONS
            electron_maxstep = 200
                    conv_thr = 1.0D-7
              diago_thr_init = 1e-4
                 startingpot = 'atomic'
                 startingwfc = 'atomic'
                 mixing_mode = 'plain'
                 mixing_beta = 0.5
                 mixing_ndim = 8
             diagonalization = 'david'
 /
&IONS
                ion_dynamics = 'bfgs'
 /

ATOMIC_SPECIES
  Li1+    0.0000000000  Li1+.pw86pbe-n-kjpaw_psl.1.0.0.UPF
  Mn3.5+    0.0000000000  Mn3.5+.pw86pbe-n-kjpaw_psl.1.0.0.UPF
  O2-    0.0000000000  O2-.pw86pbe-n-kjpaw_psl.1.0.0.UPF

ATOMIC_POSITIONS crystal
Li1+      0.87500000000000      0.87500000000000      0.87500000000000
Li1+      0.12500000000000      0.12500000000000      0.12500000000000
Li1+      0.87500000000000      0.37500000000000      0.37500000000000
Li1+      0.37500000000000      0.87500000000000      0.37500000000000
Li1+      0.37500000000000      0.37500000000000      0.87500000000000
Li1+      0.12500000000000      0.62500000000000      0.62500000000000
Li1+      0.62500000000000      0.12500000000000      0.62500000000000
Li1+      0.62500000000000      0.62500000000000      0.12500000000000
Mn3.5+      0.50000000000000      0.25000000000000      0.25000000000000
Mn3.5+      0.25000000000000      0.50000000000000      0.25000000000000
Mn3.5+      0.25000000000000      0.25000000000000      0.50000000000000
Mn3.5+      0.50000000000000      0.50000000000000      0.50000000000000
Mn3.5+      0.50000000000000      0.75000000000000      0.75000000000000
Mn3.5+      0.75000000000000      0.50000000000000      0.75000000000000
Mn3.5+      0.75000000000000      0.75000000000000      0.50000000000000
Mn3.5+      0.00000000000000      0.25000000000000      0.75000000000000
Mn3.5+      0.00000000000000      0.75000000000000      0.25000000000000
Mn3.5+      0.25000000000000      0.00000000000000      0.75000000000000
Mn3.5+      0.75000000000000      0.00000000000000      0.25000000000000
Mn3.5+      0.25000000000000      0.75000000000000      0.00000000000000
Mn3.5+      0.75000000000000      0.25000000000000      0.00000000000000
Mn3.5+      0.50000000000000      0.00000000000000      0.00000000000000
Mn3.5+      0.00000000000000      0.50000000000000      0.00000000000000
Mn3.5+      0.00000000000000      0.00000000000000      0.50000000000000
O2-      0.73730000000000      0.01270000000000      0.01270000000000
O2-      0.01270000000000      0.73730000000000      0.01270000000000
O2-      0.01270000000000      0.01270000000000      0.73730000000000
O2-      0.73730000000000      0.73730000000000      0.73730000000000
O2-      0.26270000000000      0.98730000000000      0.98730000000000
O2-      0.98730000000000      0.26270000000000      0.98730000000000
O2-      0.98730000000000      0.98730000000000      0.26270000000000
O2-      0.26270000000000      0.26270000000000      0.26270000000000
O2-      0.73730000000000      0.51270000000000      0.51270000000000
O2-      0.23730000000000      0.01270000000000      0.51270000000000
O2-      0.23730000000000      0.51270000000000      0.01270000000000
O2-      0.01270000000000      0.23730000000000      0.51270000000000
O2-      0.51270000000000      0.73730000000000      0.51270000000000
O2-      0.51270000000000      0.23730000000000      0.01270000000000
O2-      0.01270000000000      0.51270000000000      0.23730000000000
O2-      0.51270000000000      0.01270000000000      0.23730000000000
O2-      0.51270000000000      0.51270000000000      0.73730000000000
O2-      0.73730000000000      0.23730000000000      0.23730000000000
O2-      0.23730000000000      0.73730000000000      0.23730000000000
O2-      0.23730000000000      0.23730000000000      0.73730000000000
O2-      0.26270000000000      0.48730000000000      0.48730000000000
O2-      0.76270000000000      0.98730000000000      0.48730000000000
O2-      0.76270000000000      0.48730000000000      0.98730000000000
O2-      0.98730000000000      0.76270000000000      0.48730000000000
O2-      0.48730000000000      0.26270000000000      0.48730000000000
O2-      0.48730000000000      0.76270000000000      0.98730000000000
O2-      0.98730000000000      0.48730000000000      0.76270000000000
O2-      0.48730000000000      0.98730000000000      0.76270000000000
O2-      0.48730000000000      0.48730000000000      0.26270000000000
O2-      0.26270000000000      0.76270000000000      0.76270000000000
O2-      0.76270000000000      0.26270000000000      0.76270000000000
O2-      0.76270000000000      0.76270000000000      0.26270000000000

K_POINTS automatic
2  2  2   0 0 0

CELL_PARAMETERS
    15.57115429380366      0.00000000000000      0.00000000000000
     0.00000000000000     15.57115429380366      0.00000000000000
     0.00000000000000      0.00000000000000     15.57115429380366



Giovanni



> On 06 Jul 2015, at 20:51, max <aquiles011 at gmail.com> wrote:
> 
> Hello,
> 
> I'm confusing, I need to do some convergence test, but I don't know if I need primitive or one unit cell and how to select it.
> 
> I'm using this structure http://www.crystallography.net/cod/1513984.html <http://www.crystallography.net/cod/1513984.html>
> 
> I extracted the crystallographic translation. The cell formula units are 8, has 56 atoms.  See ATOMIC_POSITIONS bellow.
> 
> One unit cell of LiMn2O4 (spinel) has 7 atoms.
> 
> I have the following questions:
> 
> Do I need to put 7 atoms in the primitive cell or how many?
> 
> How can I select the atoms position for primitive or one unit cell?
> 
> ATOMIC_POSITIONS alat 
>    Li      0.125000000    0.125000000    0.125000000    
>    Li     -0.125000000    0.875000000    0.875000000    
>    Li      0.875000000   -0.125000000    0.875000000    
>    Li      0.875000000    0.875000000   -0.125000000    
>    Li     -0.125000000   -0.125000000   -0.125000000    
>    Li     -0.125000000    0.375000000    0.375000000    
>    Li      0.375000000    0.875000000    0.375000000    
>    Li      0.875000000    0.375000000    0.375000000    
>    Mn      0.500000000    0.500000000    0.500000000    
>    Mn     -0.500000000    1.250000000    1.250000000    
>    Mn      1.250000000   -0.500000000    1.250000000    
>    Mn      1.250000000    1.250000000   -0.500000000    
>    Mn     -0.500000000   -0.500000000   -0.500000000    
>    Mn      0.500000000   -0.250000000   -0.250000000    
>    Mn     -0.250000000    0.500000000   -0.250000000    
>    Mn     -0.250000000   -0.250000000    0.500000000    
>    Mn     -0.500000000    0.750000000    0.750000000    
>    Mn      0.000000000    1.250000000    0.750000000    
>    Mn      0.000000000    0.750000000    1.250000000    
>    Mn      1.250000000    0.000000000    0.750000000    
>    Mn      0.750000000   -0.500000000    0.750000000    
>    Mn      0.750000000    0.000000000    1.250000000    
>    Mn      1.250000000    0.750000000    0.000000000    
>    Mn      0.750000000    1.250000000    0.000000000    
>     O     -0.262700000    1.012700000    1.012700000    
>     O      1.012700000   -0.262700000    1.012700000    
>     O      1.012700000    1.012700000   -0.262700000    
>     O     -0.262700000   -0.262700000   -0.262700000    
>     O      0.262700000   -0.012700000   -0.012700000    
>     O     -0.012700000    0.262700000   -0.012700000    
>     O     -0.012700000   -0.012700000    0.262700000    
>     O      0.262700000    0.262700000    0.262700000    
>     O     -0.262700000    0.512700000    0.512700000    
>     O      0.237300000    1.012700000    0.512700000    
>     O      0.237300000    0.512700000    1.012700000    
>     O      1.012700000    0.237300000    0.512700000    
>     O      0.512700000   -0.262700000    0.512700000    
>     O      0.512700000    0.237300000    1.012700000    
>     O      1.012700000    0.512700000    0.237300000    
>     O      0.512700000    1.012700000    0.237300000    
>     O      0.512700000    0.512700000   -0.262700000    
>     O     -0.262700000    0.237300000    0.237300000    
>     O      0.237300000   -0.262700000    0.237300000    
>     O      0.237300000    0.237300000   -0.262700000    
>     O      0.262700000    0.487300000    0.487300000    
>     O      0.762700000   -0.012700000    0.487300000    
>     O      0.762700000    0.487300000   -0.012700000    
>     O     -0.012700000    0.762700000    0.487300000    
>     O      0.487300000    0.262700000    0.487300000    
>     O      0.487300000    0.762700000   -0.012700000    
>     O     -0.012700000    0.487300000    0.762700000    
>     O      0.487300000   -0.012700000    0.762700000    
>     O      0.487300000    0.487300000    0.262700000    
>     O      0.262700000    0.762700000    0.762700000    
>     O      0.762700000    0.262700000    0.762700000    
>     O      0.762700000    0.762700000    0.262700000
> 
> -- 
> Máximo Ramírez
> Physics Degree
> Universidad Autónoma de Santo Domingo
> _______________________________________________
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> Pw_forum at pwscf.org
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-- 

Giovanni Cantele, PhD
CNR-SPIN
c/o Dipartimento di Fisica
Universita' di Napoli "Federico II"
Complesso Universitario M. S. Angelo - Ed. 6
Via Cintia, I-80126, Napoli, Italy
e-mail: giovanni.cantele at spin.cnr.it
Phone: +39 081 676910
Skype contact: giocan74

ResearcherID: http://www.researcherid.com/rid/A-1951-2009
Web page: http://people.na.infn.it/~cantele

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