[Pw_forum] (no subject)

Ari P Seitsonen Ari.P.Seitsonen at iki.fi
Mon Apr 20 17:07:45 CEST 2015


Dear D Sakthivel,

   Adding to Giuseppe's answer about the cut-off energy, some side notes: 
Your value for 'degauss' is large - did you realise that the units are Ry, 
not eV (I often use 0.05 eV, but 0.05 Ry would be huge), plus your 
convergence criterion for the electronic structure is quite loose (10^-5), 
combined with the low cut-off energy the stress in the first configuration 
had very large components, and thus the change in the lattice constant was 
very large (components from 0.5 to 0.432690878). Is the (practically) 
non-magnetic electronic ground state correct, or maybe due to the large 
broadening of the occupation numbers?

     Greetings from Sunny Montrouge,

        apsi

-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-
   Ari Paavo Seitsonen / Ari.P.Seitsonen at iki.fi / http://www.iki.fi/~apsi/
   Ecole Normale Supérieure (ENS), Département de Chimie, Paris
   Mobile (F) : +33 789 37 24 25    (CH) : +41 79 71 90 935


On Mon, 20 Apr 2015, Giuseppe Mattioli wrote:

>
> Dear D.Sakthivel
> Your
> ecutwfc = 55
> is probably too low for your NC pseudopotentials. Try to reach convergence wrt the basis set.
> HTH
> Giuseppe
>
> On Monday, April 20, 2015 03:38:21 PM sakthivel durai wrote:
>> Dear Quantum espresso Community,
>>                      I am trying to calculate the VC- relax in my system
>> Ni2MnGa but some error...
>>   my input is...
>> &CONTROL
>>                        title = 'Ni2MnGa' ,
>>                  calculation = 'vc-relax' ,
>>                 restart_mode = 'from_scratch' ,
>>                       outdir = '/home/master/Desktop/MDS/' ,
>>                   pseudo_dir = '/home/master/Desktop/MDS 2/' ,
>>                       prefix = 'atom' ,
>>                      tstress = .false. ,
>>                      tprnfor = .false. ,
>>  /
>>  &SYSTEM
>>                        ibrav = 2,
>>                            A = 5.666 ,
>>                          nat = 4,
>>                         ntyp = 3,
>>                      ecutwfc = 55 ,
>>                  occupations = 'smearing' ,
>>                      degauss = 0.05 ,
>>                     smearing = 'fermi-dirac' ,
>>                        nspin = 2 ,
>>    starting_magnetization(1) = 0.5,
>>    starting_magnetization(2) = 0.4,
>>    starting_magnetization(3) = 0.2,
>>  /
>>  &ELECTRONS
>>             electron_maxstep = 150,
>>                     conv_thr = 1.0d-5 ,
>>                  mixing_beta = 0.7 ,
>>  /
>>  &IONS
>>                 ion_dynamics = 'bfgs' ,
>>  /
>>  &CELL
>>                cell_dynamics = 'bfgs' ,
>>  /
>> ATOMIC_SPECIES
>>    Ni   58.69300  Ni.pbe-mt_fhi.UPF
>>    Mn   54.93800  Mn.pbe-mt_fhi.UPF
>>    Ga   69.72300  Ga.pbe-mt_fhi.UPF
>> ATOMIC_POSITIONS crystal
>>    Ni      0.250000000    0.250000000    0.250000000    1  1  1
>>    Ni      0.750000000    0.750000000    0.750000000    1  1  1
>>    Mn      0.500000000    0.500000000    0.500000000    1  1  1
>>    Ga      0.000000000    0.000000000    0.000000000    1  1  1
>> K_POINTS automatic
>>   8 8 8   0 0 0

...

>>
>>      total magnetization       =     0.07 Bohr mag/cell
>>      absolute magnetization    =     0.15 Bohr mag/cell
>>
>>      iteration # 20     ecut=    55.00 Ry     beta=0.70
>>      Davidson diagonalization with overlap
>>      ethr =  4.02E-08,  avg # of iterations =  5.3
>>
>>      Magnetic moment per site:
>>      atom:    1    charge:    8.6990    magn:   -0.0020    constr:    0.0000
>>      atom:    2    charge:    8.6990    magn:   -0.0020    constr:    0.0000
>>      atom:    3    charge:    5.3367    magn:    0.0101    constr:    0.0000
>>      atom:    4    charge:    1.3950    magn:   -0.0000    constr:    0.0000
>>
>>      total cpu time spent up to now is      208.9 secs
>>
>>      End of self-consistent calculation
>>
>>  ------ SPIN UP ------------
>>
>>
>>           k = 0.0000 0.0000 0.0000 (  2085 PWs)   bands (ev):
>>
>>      2.5755   9.8135   9.8135   9.8135  10.0780  10.0780  11.4746  11.4746
>>     11.4746  12.5730  12.5730  12.8276  12.8276  12.8276  14.1243  14.1243
>>     18.7623  18.7623  18.7623
>>

...

>>
>>      6.2481   8.3987   8.3987   9.5804  10.6357  10.8539  10.8539  11.1442
>>     11.3001  11.3001  11.7780  11.8571  13.0055  13.0055  13.8067  13.8067
>>     14.0206  14.2072  14.2265
>>
>>  ------ SPIN DOWN ----------
>>
>>
>>           k = 0.0000 0.0000 0.0000 (  2085 PWs)   bands (ev):
>>
>>      2.5742   9.8105   9.8105   9.8105  10.0718  10.0718  11.4871  11.4871
>>     11.4871  12.5686  12.5686  12.8383  12.8383  12.8383  14.1056  14.1056
>>     18.7605  18.7605  18.7605
>>

...

>>
>>           k =-0.5000-1.0000 0.0000 (  2148 PWs)   bands (ev):
>>
>>      6.2458   8.3985   8.3985   9.5795  10.6301  10.8529  10.8529  11.1507
>>     11.2983  11.2983  11.7750  11.8532  13.0031  13.0031  13.8315  13.8315
>>     14.0032  14.2059  14.2341
>>
>>      the Fermi energy is    13.9712 ev
>>
>> !    total energy              =    -171.60258466 Ry
>>      Harris-Foulkes estimate   =    -171.60258537 Ry
>>      estimated scf accuracy    <       0.00000222 Ry
>>
>>      The total energy is the sum of the following terms:
>>
>>      one-electron contribution =     -13.16491140 Ry
>>      hartree contribution      =      39.95596738 Ry
>>      xc contribution           =     -32.88188265 Ry
>>      ewald contribution        =    -165.06519892 Ry
>>      smearing contrib. (-TS)   =      -0.44655907 Ry
>>
>>      total magnetization       =     0.01 Bohr mag/cell
>>      absolute magnetization    =     0.02 Bohr mag/cell
>>
>>      convergence has been achieved in  20 iterations
>>
>>      Forces acting on atoms (Ry/au):
>>
>>      atom    1 type  1   force =    -0.00000000    0.00000000    0.00000000
>>      atom    2 type  1   force =     0.00000000   -0.00000000    0.00000000
>>      atom    3 type  2   force =    -0.00000000   -0.00000000    0.00000000
>>      atom    4 type  3   force =     0.00000000    0.00000000   -0.00000000
>>
>>      Total force =     0.000000     Total SCF correction =     0.000000
>>
>>
>>      entering subroutine stress ...
>>
>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>> -792.12
>>   -0.00538473   0.00000000  -0.00000000       -792.12      0.00     -0.00
>>    0.00000000  -0.00538473   0.00000000          0.00   -792.12      0.00
>>   -0.00000000   0.00000000  -0.00538473         -0.00      0.00   -792.12
>>
>>
>>      BFGS Geometry Optimization
>>
>>      number of scf cycles    =   1
>>      number of bfgs steps    =   0
>>
>>      enthalpy new            =    -171.6025846550 Ry
>>
>>      new trust radius        =       0.4716469996 bohr
>>      new conv_thr            =       0.0000100000 Ry
>>
>>      new unit-cell volume =    198.87928 a.u.^3 (    29.47087 Ang^3 )
>>
>> CELL_PARAMETERS (alat= 10.70718827)
>>   -0.432690878   0.000000000   0.432690878
>>   -0.000000000   0.432690878   0.432690878
>>   -0.432690878   0.432690878   0.000000000
>>
>> ATOMIC_POSITIONS (crystal)
>> Ni       0.250000000   0.250000000   0.250000000
>> Ni       0.750000000   0.750000000   0.750000000
>> Mn       0.500000000   0.500000000   0.500000000
>> Ga      -0.000000000  -0.000000000   0.000000000
>>
>>
>>
>>      Writing output data file atom.save
>>      Check: negative starting charge=(component1):   -0.004425
>>      NEW-OLD atomic charge density approx. for the potential
>>
>>      negative rho (up, down):  1.881E+01 1.882E+01
>>
>>      total cpu time spent up to now is      217.0 secs
>>
>>      per-process dynamical memory:    60.0 Mb
>>
>>      Self-consistent Calculation
>>
>>      iteration #  1     ecut=    55.00 Ry     beta=0.70
>>      Davidson diagonalization with overlap
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  2 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  1 eigenvalues not converged
>>      c_bands:  2 eigenvalues not converged
>>      ethr =  1.00E-06,  avg # of iterations = 18.2
>>
>>      negative rho (up, down):  3.229E+00 3.231E+00
>>
>>      Magnetic moment per site:
>>      atom:    1    charge:    5.4206    magn:    0.0015    constr:    0.0000
>>      atom:    2    charge:    5.4206    magn:    0.0015    constr:    0.0000
>>      atom:    3    charge:    0.7461    magn:    0.0013    constr:    0.0000
>>      atom:    4    charge:    0.2023    magn:   -0.0000    constr:    0.0000
>>
>>      total cpu time spent up to now is      249.8 secs
>>
>>      WARNING: integrated charge=    17.62834225, expected=    30.00000000
>>
>>  %%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%
>>      Error in routine electrons (1):
>>      charge is wrong
>>  %%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%
>>
>>      stopping ...
>>
>>      thank you...
>>  D.Sakthivel.
>> M Phil student
>> Madurai Kamaraj University.
>> Madurai.
>> Tamil Nadu.
>> India.
>
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>
>   Giuseppe Mattioli
>   CNR - ISTITUTO DI STRUTTURA DELLA MATERIA
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>
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