[Pw_forum] scf convergence is hard to reach with DFT+U+SOC using QE5.0

Fpzheng fpzheng2013 at pku.edu.cn
Sun Jun 8 18:45:33 CEST 2014


Dear all
Hi,
I  face a serious problem  that the convergence  of scf calculation  is hard to reach  in the calculation of  DFT+U and Spin Orbit Coupling.
I  greatly  appreciate to give me some suggestions to deal with my problem.

Thanks in advance!

Feipeng Zheng
PHD students of Peking University, China

My input file and the information about convergence are listed below:


(1)Input
~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~
&control
   prefix = 'cn'
   calculation = 'scf'
   restart_mode = 'from_scratch'
    wf_collect = .false.
   tstress = .true.
   tprnfor = .true.
   outdir = './outdir'
   wfcdir = './wfcdir'
   pseudo_dir = './'

/
&system
   ibrav = -12
   A=5.4270000458 
   B=9.3950004578
   C=5.614
   cosAB=0
   cosBC=0
   cosAC=-0.3261786758
   nat = 24
   ntyp = 4
   nbnd = 216
   ecutwfc = 60.0
   occupations  =  'smearing' ,
                    smearing  =  'gaussian' ,
                     degauss  =  0.01 ,
     lda_plus_u  = .true., 
     lda_plus_u_kind = 1, 
    Hubbard_U(1)=1.7 , Hubbard_U(2)=1.7 ,Hubbard_J(1,1)=0.6, Hubbard_J(1,2)=0.6
    lspinorb=.true.,  noncolin=.true., 
    starting_magnetization(1)=0.5, starting_magnetization(2)=-0.5, starting_magnetization(3)=0, starting_magnetization(4)=0
/
&electrons
   electron_maxstep = 200
   conv_thr = 1.0d-6
   mixing_mode = 'plain'
   mixing_beta = 0.3
   mixing_ndim = 8
   diagonalization = 'david'
   diago_david_ndim = 4
/
ATOMIC_SPECIES
  Ir1 192.217  Ir.rel-pbesol-n-rrkjus_psl.0.2.3.UPF
  Ir2 192.217  Ir.rel-pbesol-n-rrkjus_psl.0.2.3.UPF
  Na  22.98977 Na.rel-pbesol-spn-rrkjus_psl.0.2.UPF
  O   15.9994  O.rel-pbesol-n-rrkjus_psl.0.1.UPF
ATOMIC_POSITIONS crystal
 Ir1    0.500000000         0.166999996         0.000000000
 Ir1    0.000000000         0.333000004         0.000000000
 Ir2    0.500000000         0.833000004         0.000000000
 Ir2    0.000000000         0.666999996         0.000000000
 Na    0.000000000         0.000000000         0.000000000
 Na    0.500000000         0.500000000         0.000000000
 Na    0.500000000         0.000000000         0.500000000
 Na    0.000000000         0.500000000         0.500000000
 Na    0.500000000         0.340000004         0.500000000
 Na    0.500000000         0.659999967         0.500000000
 Na    0.000000000         0.840000033         0.500000000
 Na    0.000000000         0.159999996         0.500000000
 O    0.748000026         0.178000003         0.788999975
 O    0.251999974         0.822000027         0.211000025
 O    0.251999974         0.178000003         0.211000025
 O    0.748000026         0.822000027         0.788999975
 O    0.248000026         0.677999973         0.788999975
 O    0.751999974         0.321999997         0.211000025
 O    0.751999974         0.677999973         0.211000025
 O    0.248000026         0.321999997         0.788999975
 O    0.711000025         0.000000000         0.203999996
 O    0.288999975         0.000000000         0.796000004
 O    0.211000025         0.500000000         0.203999996
 O    0.788999975         0.500000000         0.796000004
K_POINTS automatic
6 3 6 1 1 1
 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~
(2)Information about the convergence

     estimated scf accuracy    <       5.92167692 Ry
     estimated scf accuracy    <       0.97254388 Ry
     estimated scf accuracy    <       0.22957473 Ry
     estimated scf accuracy    <       0.05303115 Ry
     estimated scf accuracy    <       0.01821857 Ry
     estimated scf accuracy    <       0.01087345 Ry
     estimated scf accuracy    <       0.00752675 Ry
     estimated scf accuracy    <       0.00439903 Ry
     estimated scf accuracy    <       0.00976111 Ry
     estimated scf accuracy    <       0.00971859 Ry
     estimated scf accuracy    <       0.00379758 Ry
     estimated scf accuracy    <       0.00549082 Ry
     estimated scf accuracy    <       0.00292167 Ry
     estimated scf accuracy    <       0.00297945 Ry
     estimated scf accuracy    <       0.00296944 Ry
     estimated scf accuracy    <       0.00357511 Ry
     estimated scf accuracy    <       0.01859299 Ry
     estimated scf accuracy    <       0.01614578 Ry
     estimated scf accuracy    <       0.00284335 Ry
     estimated scf accuracy    <       0.00220986 Ry
     estimated scf accuracy    <       0.00199116 Ry
     estimated scf accuracy    <       0.00394812 Ry
     estimated scf accuracy    <       0.00187060 Ry
     estimated scf accuracy    <       0.00109610 Ry
     estimated scf accuracy    <       0.00136364 Ry
     estimated scf accuracy    <       0.00148185 Ry
     estimated scf accuracy    <       0.00149291 Ry
     estimated scf accuracy    <       0.00128022 Ry
     estimated scf accuracy    <       0.00126421 Ry
     estimated scf accuracy    <       0.00119635 Ry
     estimated scf accuracy    <       0.00154749 Ry
     estimated scf accuracy    <       0.00087598 Ry
     estimated scf accuracy    <       0.00177820 Ry
     estimated scf accuracy    <       0.00173430 Ry
     estimated scf accuracy    <       0.00212876 Ry
     estimated scf accuracy    <       0.00153512 Ry
     estimated scf accuracy    <       0.00131154 Ry
     estimated scf accuracy    <       0.00139106 Ry
     estimated scf accuracy    <       0.00202859 Ry
     estimated scf accuracy    <       0.00183535 Ry
     estimated scf accuracy    <       0.00110236 Ry
     estimated scf accuracy    <       0.00125853 Ry
     estimated scf accuracy    <       0.00114915 Ry
     estimated scf accuracy    <       0.00165795 Ry
     estimated scf accuracy    <       0.00070753 Ry
     estimated scf accuracy    <       0.00103440 Ry
     estimated scf accuracy    <       0.00076983 Ry
     estimated scf accuracy    <       0.00106630 Ry
     estimated scf accuracy    <       0.00138150 Ry
     estimated scf accuracy    <       0.00135628 Ry
     estimated scf accuracy    <       0.00139915 Ry
     estimated scf accuracy    <       0.00081134 Ry
     estimated scf accuracy    <       0.00133499 Ry
     estimated scf accuracy    <       0.00158556 Ry
     estimated scf accuracy    <       0.00161960 Ry
     estimated scf accuracy    <       0.00244889 Ry
     estimated scf accuracy    <       0.00166725 Ry
     estimated scf accuracy    <       0.00116166 Ry
     estimated scf accuracy    <       0.00171726 Ry
     estimated scf accuracy    <       0.00207491 Ry
     estimated scf accuracy    <       0.00207093 Ry
     estimated scf accuracy    <       0.00175628 Ry
     estimated scf accuracy    <       0.00173412 Ry
     estimated scf accuracy    <       0.00170433 Ry
     estimated scf accuracy    <       0.00257291 Ry
     estimated scf accuracy    <       0.00199391 Ry
     estimated scf accuracy    <       0.00193952 Ry
     estimated scf accuracy    <       0.00126945 Ry
     estimated scf accuracy    <       0.00125673 Ry
     estimated scf accuracy    <       0.00157669 Ry
     estimated scf accuracy    <       0.00227168 Ry
     estimated scf accuracy    <       0.00152062 Ry
     estimated scf accuracy    <       0.00120945 Ry
     estimated scf accuracy    <       0.00156651 Ry
     estimated scf accuracy    <       0.00143003 Ry
     estimated scf accuracy    <       0.00160748 Ry
     estimated scf accuracy    <       0.00118836 Ry
     estimated scf accuracy    <       0.00122127 Ry
     estimated scf accuracy    <       0.00120106 Ry
     estimated scf accuracy    <       0.00130648 Ry
     estimated scf accuracy    <       0.00136426 Ry
     estimated scf accuracy    <       0.00122502 Ry
     estimated scf accuracy    <       0.00108343 Ry
     estimated scf accuracy    <       0.00265258 Ry
     estimated scf accuracy    <       0.00159231 Ry
     estimated scf accuracy    <       0.00161320 Ry
     estimated scf accuracy    <       0.00260174 Ry
     estimated scf accuracy    <       0.00144941 Ry
     estimated scf accuracy    <       0.00233780 Ry
     estimated scf accuracy    <       0.00184648 Ry
     estimated scf accuracy    <       0.00132588 Ry
     estimated scf accuracy    <       0.00134312 Ry
     estimated scf accuracy    <       0.00209603 Ry
     estimated scf accuracy    <       0.00163010 Ry
     estimated scf accuracy    <       0.00135211 Ry
     estimated scf accuracy    <       0.00140337 Ry
     estimated scf accuracy    <       0.00312293 Ry
     estimated scf accuracy    <       0.00176500 Ry
     estimated scf accuracy    <       0.00268589 Ry
     estimated scf accuracy    <       0.00249467 Ry
     estimated scf accuracy    <       0.00185384 Ry
     estimated scf accuracy    <       0.00217734 Ry
     estimated scf accuracy    <       0.00245582 Ry
     estimated scf accuracy    <       0.00263931 Ry
     estimated scf accuracy    <       0.00214840 Ry
     estimated scf accuracy    <       0.00271914 Ry
     estimated scf accuracy    <       0.00272293 Ry
     estimated scf accuracy    <       0.00298563 Ry
     estimated scf accuracy    <       0.00203851 Ry
     estimated scf accuracy    <       0.00216732 Ry
     estimated scf accuracy    <       0.00206684 Ry
     estimated scf accuracy    <       0.00200724 Ry
     estimated scf accuracy    <       0.00224128 Ry
     estimated scf accuracy    <       0.00211667 Ry
     estimated scf accuracy    <       0.00197926 Ry
     estimated scf accuracy    <       0.00278075 Ry
     estimated scf accuracy    <       0.00333196 Ry
     estimated scf accuracy    <       0.00381661 Ry
     estimated scf accuracy    <       0.00543998 Ry
     estimated scf accuracy    <       0.00134101 Ry
     estimated scf accuracy    <       0.00277809 Ry
     estimated scf accuracy    <       0.00150992 Ry
     estimated scf accuracy    <       0.00186318 Ry
     estimated scf accuracy    <       0.00211254 Ry
     estimated scf accuracy    <       0.00230520 Ry
     estimated scf accuracy    <       0.00370439 Ry
     estimated scf accuracy    <       0.00280689 Ry
     estimated scf accuracy    <       0.00329003 Ry
     estimated scf accuracy    <       0.00212648 Ry
     estimated scf accuracy    <       0.00252098 Ry
     estimated scf accuracy    <       0.00208129 Ry
     estimated scf accuracy    <       0.00248616 Ry
     estimated scf accuracy    <       0.00285185 Ry
     estimated scf accuracy    <       0.00380639 Ry
     estimated scf accuracy    <       0.00595663 Ry
     estimated scf accuracy    <       0.00609239 Ry
     estimated scf accuracy    <       0.00361332 Ry
     estimated scf accuracy    <       0.00378039 Ry
     estimated scf accuracy    <       0.00298567 Ry
     estimated scf accuracy    <       0.00335279 Ry
     estimated scf accuracy    <       0.00249541 Ry
     estimated scf accuracy    <       0.00404341 Ry
     estimated scf accuracy    <       0.00366412 Ry
     estimated scf accuracy    <       0.00417476 Ry
     estimated scf accuracy    <       0.00352050 Ry
     estimated scf accuracy    <       0.01228127 Ry
     estimated scf accuracy    <       0.00297789 Ry
     estimated scf accuracy    <       0.00405888 Ry
     estimated scf accuracy    <       0.00385294 Ry
     estimated scf accuracy    <       0.00480060 Ry
     estimated scf accuracy    <       0.00496324 Ry
     estimated scf accuracy    <       0.00415109 Ry
     estimated scf accuracy    <       0.00296269 Ry
     estimated scf accuracy    <       0.00300026 Ry
     estimated scf accuracy    <       0.00499471 Ry
     estimated scf accuracy    <       0.00336766 Ry
     estimated scf accuracy    <       0.00349984 Ry
     estimated scf accuracy    <       0.00528050 Ry
     estimated scf accuracy    <       0.00362642 Ry
     estimated scf accuracy    <       0.00364593 Ry
     estimated scf accuracy    <       0.00533317 Ry
     estimated scf accuracy    <       0.00348740 Ry
     estimated scf accuracy    <       0.00489642 Ry
     estimated scf accuracy    <       0.02135842 Ry
     estimated scf accuracy    <       0.00341085 Ry
     estimated scf accuracy    <       0.00718359 Ry
     estimated scf accuracy    <       0.00377118 Ry
     estimated scf accuracy    <       0.02611920 Ry
     estimated scf accuracy    <       0.00336025 Ry
     estimated scf accuracy    <       0.00411045 Ry
     estimated scf accuracy    <       0.00334764 Ry
     estimated scf accuracy    <       0.00368985 Ry
     estimated scf accuracy    <       0.00319746 Ry
     estimated scf accuracy    <       0.00965470 Ry
     estimated scf accuracy    <       0.00685133 Ry
     estimated scf accuracy    <       0.00442885 Ry
     estimated scf accuracy    <       0.00397514 Ry
     estimated scf accuracy    <       0.01779225 Ry
     estimated scf accuracy    <       0.00572820 Ry
     estimated scf accuracy    <       0.00550507 Ry
     estimated scf accuracy    <       0.00554672 Ry
     estimated scf accuracy    <       0.00374998 Ry
     estimated scf accuracy    <       0.00729374 Ry
     estimated scf accuracy    <       0.00522458 Ry



__________________________________________________
Feipeng Zheng
 
International Center For Quantum Materials, Peking University
 
TEL:15652969449   




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