[Pw_forum] vc-relax of a 60 atom supercell

Elie Moujaes elie.moujaes at hotmail.co.uk
Mon Jun 7 22:19:33 CEST 2010


Dear all, I am trying to relax a 60 atom supercell of graphene using vc-relax. 

 

(1) I want the relaxation to be with respect to both atomic coordinates and supercell vectors, Is vc-relax the correct calculation to use.

 

(2) I used a vc relax to my superstructure but  the programm stopped at the 9th iteration (well it did not stop literally but the calculations ended with no 9th iterations and no converged results along with errors related to the c_bands):

 

Initial potential from superposition of free atoms
     Check: negative starting charge=   -1.223428

     starting charge  239.99756, renormalised to  240.00000

     negative rho (up, down):  0.122E+01 0.000E+00
     Starting wfc are  240 atomic wfcs

     total cpu time spent up to now is  11871.45 secs

     per-process dynamical memory:   384.3 Mb

     Self-consistent Calculation

     iteration #  1     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     ethr =  1.00E-02,  avg # of iterations =  6.7

     negative rho (up, down):  0.117E+01 0.000E+00

     total cpu time spent up to now is  47489.34 secs

     total energy              =    -643.54940490 Ry
     Harris-Foulkes estimate   =    -643.62010992 Ry
     estimated scf accuracy    <       4.23960826 Ry

     iteration #  2     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     ethr =  1.77E-03,  avg # of iterations =  2.2

     negative rho (up, down):  0.109E+00 0.000E+00

     total cpu time spent up to now is  64468.90 secs

     total energy              =    -642.58636317 Ry
     Harris-Foulkes estimate   =    -643.55371202 Ry
     estimated scf accuracy    <       3.93330724 Ry

     iteration #  3     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     ethr =  1.64E-03,  avg # of iterations =  2.0

     negative rho (up, down):  0.148E+00 0.000E+00

     total cpu time spent up to now is  85947.86 secs

     total energy              =    -642.70459925 Ry
     Harris-Foulkes estimate   =    -642.70343771 Ry
     estimated scf accuracy    <       0.07850650 Ry

     iteration #  4     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     ethr =  3.27E-05,  avg # of iterations = 12.4

     negative rho (up, down):  0.151E+00 0.000E+00

     total cpu time spent up to now is 112929.09 secs

     total energy              =    -642.71219905 Ry
     Harris-Foulkes estimate   =    -642.71283310 Ry
     estimated scf accuracy    <       0.06999785 Ry

     iteration #  5     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     ethr =  2.92E-05,  avg # of iterations =  1.1

     negative rho (up, down):  0.349E+00 0.000E+00

     total cpu time spent up to now is 135493.02 secs

     total energy              =    -642.68724348 Ry
     Harris-Foulkes estimate   =    -642.71241729 Ry
     estimated scf accuracy    <       0.06752485 Ry

     iteration #  6     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     ethr =  2.81E-05,  avg # of iterations =  8.8

     negative rho (up, down):  0.397E+00 0.000E+00

     total cpu time spent up to now is 167131.43 secs

     total energy              =    -642.68305797 Ry
     Harris-Foulkes estimate   =    -642.69027767 Ry
     estimated scf accuracy    <       0.02138677 Ry

     iteration #  7     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     c_bands:  1 eigenvalues not converged
     c_bands:  1 eigenvalues not converged
     ethr =  8.91E-06,  avg # of iterations =  9.6

     negative rho (up, down):  0.375E+00 0.000E+00

     total cpu time spent up to now is 195521.38 secs

     total energy              =    -642.68507799 Ry
     Harris-Foulkes estimate   =    -642.68373726 Ry
     estimated scf accuracy    <       0.01412971 Ry

     iteration #  8     ecut=    10.00 Ry     beta=0.05
     Davidson diagonalization with overlap
     ethr =  5.89E-06,  avg # of iterations =  1.2

     negative rho (up, down):  0.241E+00 0.000E+00

     total cpu time spent up to now is 217886.22 secs

     total energy              =    -642.68307655 Ry
     Harris-Foulkes estimate   =    -642.68513864 Ry
     estimated scf accuracy    <       0.01367803 Ry

     iteration #  9     ecut=    10.00 Ry     beta=0.05
 
The input file is:

 

 

&control
    prefix='GB mgraphene',
    calculation='vc-relax',
    restart_mode='from_scratch',
    pseudo_dir = '/exp/home/caiapo/emoujaes/espresso/espresso-4.1.3/pseudo/',
    outdir='/exp/home/caiapo/emoujaes/Moujaes-Results/',
    tstress = .true.,
    tprnfor = .true.,
    disk_io = 'low'
      
 /
 &system    
    ibrav=  0, celldm(1) =1.88972, nat=60, ntyp= 1, ecutwfc = 110D0 ,occupations='smearing', smearing='methfessel-paxton', degauss=0.01
/
 &electrons
    conv_thr=1.D-8,     
    mixing_beta=0.05D0,
    mixing_mode='local-TF',
    diagonalization='david' 
 /
  & ions
    ion_dynamics = 'bfgs',
    pot_extrapolation = 'second-order',
    wfc_extrapolation = 'second-order'
/
  & cell
    cell_dynamics = 'bfgs',
    press_conv_thr = 0.1
 
ATOMIC_SPECIES
 C  12.0107  C.pz-vbc.UPF
ATOMIC_POSITIONS angstrom
 C   -11.737980    -3.561278     0.000000
 C   -11.057718    -1.211571     0.000000
 C   -12.450000    -7.189838     0.000000
 C   -12.450000    -5.773759     0.000000

.....................

(up to the remainder of the 60 atoms)

 

K_POINTS automatic
26 26 1 0 0 0
 
CELL_PARAMETERS hexagonal
 
24.527679   0.000000    0.000000
0.000003    6.614491    0.000000
0.000000    0.000000   10.000000
 
 		 	   		  
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