[Pw_forum] vc-relax - Convergence Problems

Stefano de Gironcoli degironc at sissa.it
Fri Aug 20 21:06:01 CEST 2010


so far so good...  maybe it's only slow...
I don't recall now exactly how BFGS works but the fact that at each stem 
it says

enthalpy_new < enthalpy_old

maybe means that it's going downhill without finding a minimum along the 
line search and the step is limited by the trust_radius.
maybe you started very far  from the  minimum or there are rotations of 
some rigid units involved ...

stefano

Andre Martinotto wrote:
> Yes, the enthalpy is decreasing the enthalpy is decreasing. Below the values
> of the  enthaply.
>
> Best regards,
> André Luis Martinotto
>
> Andre Martinotto
> Email: almartinotto at gmail.com
> Computing Department
> Universidade de Caxias do Sul
> Caxias do Sul - RS, Brazil
>
>      enthalpy old            =   -1018.4377035275 Ry
>      enthalpy new            =   -1018.4494900797 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4494900797 Ry
>      enthalpy new            =   -1018.4568547798 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4568547798 Ry
>      enthalpy new            =   -1018.4624673172 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4624673172 Ry
>      enthalpy new            =   -1018.4675637420 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4675637420 Ry
>      enthalpy new            =   -1018.4745374801 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4745374801 Ry
>      enthalpy new            =   -1018.4787658712 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4787658712 Ry
>      enthalpy new            =   -1018.4839453395 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4839453395 Ry
>      enthalpy new            =   -1018.4906317150 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4906317150 Ry
>      enthalpy new            =   -1018.4927767110 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4927767110 Ry
>      enthalpy new            =   -1018.4939707446 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4939707446 Ry
>      enthalpy new            =   -1018.4946012005 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4946012005 Ry
>      enthalpy new            =   -1018.4951369286 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4951369286 Ry
>      enthalpy new            =   -1018.4955690712 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4955690712 Ry
>      enthalpy new            =   -1018.4961210855 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4961210855 Ry
>      enthalpy new            =   -1018.4964627786 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4964627786 Ry
>      enthalpy new            =   -1018.4971749436 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4971749436 Ry
>      enthalpy new            =   -1018.4985789257 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4985789257 Ry
>      enthalpy new            =   -1018.4996031008 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.4996031008 Ry
>      enthalpy new            =   -1018.5008017865 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5008017865 Ry
>      enthalpy new            =   -1018.5036232518 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5036232518 Ry
>      enthalpy new            =   -1018.5070595112 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5070595112 Ry
>      enthalpy new            =   -1018.5117630729 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5117630729 Ry
>      enthalpy new            =   -1018.5170591719 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5170591719 Ry
>      enthalpy new            =   -1018.5222913399 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5222913399 Ry
>      enthalpy new            =   -1018.5282241124 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5282241124 Ry
>      enthalpy new            =   -1018.5342597827 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5342597827 Ry
>      enthalpy new            =   -1018.5406966898 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5406966898 Ry
>      enthalpy new            =   -1018.5469217329 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5469217329 Ry
>      enthalpy new            =   -1018.5530869862 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5530869862 Ry
>      enthalpy new            =   -1018.5599277199 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5599277199 Ry
>      enthalpy new            =   -1018.5668277117 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5668277117 Ry
>      enthalpy new            =   -1018.5740583719 Ry
>      CASE: enthalpy_new < enthalpy_old
>      enthalpy old            =   -1018.5740583719 Ry
>      enthalpy new            =   -1018.5816796313 Ry
>
> **
> On Fri, Aug 20, 2010 at 2:53 PM, Stefano de Gironcoli <degironc at sissa.it>wrote:
>
>   
>> is the enthalpy decreasing during the relaxation ?
>> stefano
>>
>> Andre Martinotto wrote:
>>     
>>> Dear Stefano,
>>>
>>> Sorry.  I sent the wrong input file. The outputs correspond to the file
>>> below.
>>>
>>> Best regards,
>>> André Luis Martinotto
>>>
>>> Andre Martinotto
>>> Email: almartinotto at gmail.com
>>> Computing Department
>>> Universidade de Caxias do Sul
>>> Caxias do Sul - RS, Brazil
>>>
>>> &CONTROL
>>>                        title = CoSb3 ,
>>>                  calculation = 'vc-relax',
>>>                 restart_mode = 'restart',
>>>                   wf_collect = .true. ,
>>>                       outdir = '/dados/almartin/est2_a' ,
>>>                       wfcdir = '/dados/almartin/est2_a' ,
>>>                   pseudo_dir = '/home/u/almartin/cosb3/pseudo' ,
>>>                       prefix = 'est1' ,
>>>                etot_conv_thr = 1.0D-4 ,
>>>                forc_conv_thr = 1.0D-3 ,
>>>                      tstress = .true. ,
>>>                      tprnfor = .true.
>>>  /
>>>  &SYSTEM
>>>                        ibrav = 1,
>>>                            A = 8.5012 ,
>>>                          nat = 32,
>>>                         ntyp = 2,
>>>                      ecutwfc = 30. ,
>>>                      ecutrho = 300 ,
>>>                      input_dft = 'PBE' ,
>>>                  occupations = 'smearing' ,
>>>                      degauss = 0.01 ,
>>>                     smearing = 'marzari-vanderbilt' ,
>>>  /
>>>  &ELECTRONS
>>>                     conv_thr = 1.0D-9 ,
>>>                  startingpot = 'atomic' ,
>>>                  startingwfc = 'atomic' ,
>>>                  mixing_mode = 'plain' ,
>>>                  mixing_beta = 0.7D0 ,
>>>              diagonalization = 'david' ,
>>>  /
>>>  &IONS
>>>                 ion_dynamics = 'bfgs' ,
>>>                ion_positions = 'default' ,
>>>  /
>>>  &CELL
>>>                cell_dynamics = 'bfgs' ,
>>>                        press = 0.D0 ,
>>>               press_conv_thr = 0.2D0 ,
>>>                  cell_factor = 1.5D0 ,
>>>  /
>>> ATOMIC_SPECIES
>>>    Co   58.93300  Co.pbe-nd-rrkjus.UPF
>>>    Sb  121.76000  Sb.pbe-rrkjus.UPF
>>> ATOMIC_POSITIONS crystal
>>> Co      0.25    0.25    0.25    1 1 1
>>> Co      0.75    0.75    0.25    1 1 1
>>> Co      0.75    0.25    0.75    1 1 1
>>> Co      0.25    0.75    0.75    1 1 1
>>> Co      0.75    0.75    0.75    1 1 1
>>> Co      0.25    0.25    0.75    1 1 1
>>> Co      0.25    0.75    0.25    1 1 1
>>> Co      0.75    0.25    0.25    1 1 1
>>> Sb      0       0.6646  0.8421  1 1 1
>>> Sb      0       0.3354  0.8421  1 1 1
>>> Sb      0       0.6646  0.1579  1 1 1
>>> Sb      0       0.3354  0.1579  1 1 1
>>> Sb      0.8421  0       0.6646  1 1 1
>>> Sb      0.6646  0.8421  0       1 1 1
>>> Sb      0.8421  0       0.3354  1 1 1
>>> Sb      0.3354  0.8421  0       1 1 1
>>> Sb      0.1579  0       0.6646  1 1 1
>>> Sb      0.6646  0.1579  0       1 1 1
>>> Sb      0.1579  0       0.3354  1 1 1
>>> Sb      0.  0.  0.       0 0 0
>>> Sb      0.5     0.1646  0.3421  1 1 1
>>> Sb      0.5     0.8354  0.3421  1 1 1
>>> Sb      0.5     0.1646  0.6579  1 1 1
>>> Sb      0.5     0.8354  0.6579  1 1 1
>>> Sb      0.3421  0.5     0.1646  1 1 1
>>> Sb      0.1646  0.3421  0.5     1 1 1
>>> Sb      0.3421  0.5     0.8354  1 1 1
>>> Sb      0.8354  0.3421  0.5     1 1 1
>>> Sb      0.6579  0.5     0.1646  1 1 1
>>> Sb      0.1646  0.6579  0.5     1 1 1
>>> Sb      0.6579  0.5     0.8354  1 1 1
>>> Sb      0.5  0.5  0.5     0 0 0
>>> K_POINTS automatic
>>>   8 8 8 0 0 0
>>>
>>>
>>>
>>> On Fri, Aug 20, 2010 at 12:17 PM, Stefano de Gironcoli <
>>>       
>> degironc at sissa.it>wrote:
>>     
>>>       
>>>> you ARE NOT making a vc-relaxation unless you specify
>>>> calculation='vc-relax'
>>>> stefano
>>>>
>>>> Andre Martinotto wrote:
>>>>
>>>>         
>>>>> Dear all,
>>>>>
>>>>> I'm trying to make a vc-relax optimization of a structure with
>>>>>           
>> vacancies,
>>     
>>>>> but I'm having some problems for convergence. I have a problem with
>>>>>
>>>>>           
>>>> forces
>>>>
>>>>         
>>>>> convergence. Below the input file as are the force and stress results.
>>>>>
>>>>> Someone would have some suggestion to solve this problem?
>>>>>
>>>>> Thanks!
>>>>>
>>>>> Best regards,
>>>>> André Luis Martinotto
>>>>>
>>>>> Andre Martinotto
>>>>> Email: almartinotto at gmail.com
>>>>> Computing Department
>>>>> Universidade de Caxias do Sul
>>>>> Caxias do Sul - RS, Brazil
>>>>>
>>>>>
>>>>>
>>>>>
>>>>> /------------------------------------- input file
>>>>> ---------------------------------------/
>>>>>  &CONTROL
>>>>>                        title = CoSb3 ,
>>>>>                  calculation = 'relax',
>>>>>                 restart_mode = 'restart',
>>>>>                   wf_collect = .true. ,
>>>>>                       outdir = '/dados/almartin/est2_a' ,
>>>>>                       wfcdir = '/dados/almartin/est2_a' ,
>>>>>                   pseudo_dir = '/home/u/almartin/cosb3/pseudo' ,
>>>>>                       prefix = 'est1' ,
>>>>>                etot_conv_thr = 1.0D-4 ,
>>>>>                forc_conv_thr = 1.0D-3 ,
>>>>>                      tstress = .true. ,
>>>>>                      tprnfor = .true.
>>>>>  /
>>>>>  &SYSTEM
>>>>>                        ibrav = 1,
>>>>>                            A = 8.5012 ,
>>>>>                          nat = 32,
>>>>>                         ntyp = 2,
>>>>>                      ecutwfc = 30. ,
>>>>>                      ecutrho = 300 ,
>>>>>                      input_dft = 'PBE' ,
>>>>>                  occupations = 'smearing' ,
>>>>>                      degauss = 0.01 ,
>>>>>                     smearing = 'marzari-vanderbilt' ,
>>>>>  /
>>>>>  &ELECTRONS
>>>>>                     conv_thr = 1.0D-9 ,
>>>>>                  startingpot = 'atomic' ,
>>>>>                  startingwfc = 'atomic' ,
>>>>>                  mixing_mode = 'plain' ,
>>>>>                  mixing_beta = 0.7D0 ,
>>>>>              diagonalization = 'david' ,
>>>>>  /
>>>>>  &IONS
>>>>>                 ion_dynamics = 'bfgs' ,
>>>>>                ion_positions = 'default' ,
>>>>>  /
>>>>> &CELL
>>>>>                cell_dynamics = 'bfgs' ,
>>>>>                        press = 0.D0 ,
>>>>>               press_conv_thr = 0.2D0 ,
>>>>>                  cell_factor = 1.5D0 ,
>>>>>  /
>>>>> ATOMIC_SPECIES
>>>>>    Co   58.93300  Co.pbe-nd-rrkjus.UPF
>>>>>    Sb  121.76000  Sb.pbe-rrkjus.UPF
>>>>> ATOMIC_POSITIONS crystal
>>>>> Co      0.25    0.25    0.25    1 1 1
>>>>> Co      0.75    0.75    0.25    1 1 1
>>>>> Co      0.75    0.25    0.75    1 1 1
>>>>> Co      0.25    0.75    0.75    1 1 1
>>>>> Co      0.75    0.75    0.75    1 1 1
>>>>> Co      0.25    0.25    0.75    1 1 1
>>>>> Co      0.25    0.75    0.25    1 1 1
>>>>> Co      0.75    0.25    0.25    1 1 1
>>>>> Sb      0       0.6646  0.8421  1 1 1
>>>>> Sb      0       0.3354  0.8421  1 1 1
>>>>> Sb      0       0.6646  0.1579  1 1 1
>>>>> Sb      0       0.3354  0.1579  1 1 1
>>>>> Sb      0.8421  0       0.6646  1 1 1
>>>>> Sb      0.6646  0.8421  0       1 1 1
>>>>> Sb      0.8421  0       0.3354  1 1 1
>>>>> Sb      0.3354  0.8421  0       1 1 1
>>>>> Sb      0.1579  0       0.6646  1 1 1
>>>>> Sb      0.6646  0.1579  0       1 1 1
>>>>> Sb      0.1579  0       0.3354  1 1 1
>>>>> Sb      0.  0.  0.           0 0 0
>>>>> Sb      0.5     0.1646  0.3421  1 1 1
>>>>> Sb      0.5     0.8354  0.3421  1 1 1
>>>>> Sb      0.5     0.1646  0.6579  1 1 1
>>>>> Sb      0.5     0.8354  0.6579  1 1 1
>>>>> Sb      0.3421  0.5     0.1646  1 1 1
>>>>> Sb      0.1646  0.3421  0.5     1 1 1
>>>>> Sb      0.3421  0.5     0.8354  1 1 1
>>>>> Sb      0.8354  0.3421  0.5     1 1 1
>>>>> Sb      0.6579  0.5     0.1646  1 1 1
>>>>> Sb      0.1646  0.6579  0.5     1 1 1
>>>>> Sb      0.6579  0.5     0.8354  1 1 1
>>>>> Sb      0.5  0.5  0.5         0 0 0
>>>>> K_POINTS automatic
>>>>>   8 8 8 0 0 0
>>>>>
>>>>> /------------------------------------- stress results
>>>>> --------------------------------------/
>>>>>
>>>>>     entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.77
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 9.48
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 11.91
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 4.78
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -6.89
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -2.65
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.31
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 5.44
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 2.47
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -2.82
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -1.30
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.08
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.71
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.11
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.70
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.16
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -0.77
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -1.30
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -1.45
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -1.23
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -0.56
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.39
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.24
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.92
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 2.18
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 2.16
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.82
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 1.35
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.75
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> 0.30
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -0.03
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -0.37
>>>>>      entering subroutine stress ...
>>>>>           total   stress  (Ry/bohr**3)                   (kbar)     P=
>>>>> -0.72
>>>>>
>>>>> /------------------------------------- force results
>>>>> --------------------------------------/
>>>>>
>>>>>      Total force =     0.072779     Total SCF correction =     0.000066
>>>>>      Total force =     0.053372     Total SCF correction =     0.000053
>>>>>      Total force =     0.044120     Total SCF correction =     0.000023
>>>>>      Total force =     0.045980     Total SCF correction =     0.000024
>>>>>      Total force =     0.049875     Total SCF correction =     0.000027
>>>>>      Total force =     0.043061     Total SCF correction =     0.000055
>>>>>      Total force =     0.033627     Total SCF correction =     0.000027
>>>>>      Total force =     0.024939     Total SCF correction =     0.000032
>>>>>      Total force =     0.022018     Total SCF correction =     0.000009
>>>>>      Total force =     0.015573     Total SCF correction =     0.000049
>>>>>      Total force =     0.013346     Total SCF correction =     0.000039
>>>>>      Total force =     0.010870     Total SCF correction =     0.000017
>>>>>      Total force =     0.010344     Total SCF correction =     0.000031
>>>>>      Total force =     0.016943     Total SCF correction =     0.000021
>>>>>      Total force =     0.015429     Total SCF correction =     0.000031
>>>>>      Total force =     0.013450     Total SCF correction =     0.000013
>>>>>      Total force =     0.015799     Total SCF correction =     0.000010
>>>>>      Total force =     0.023243     Total SCF correction =     0.000032
>>>>>      Total force =     0.028594     Total SCF correction =     0.000015
>>>>>      Total force =     0.038065     Total SCF correction =     0.000030
>>>>>      Total force =     0.044262     Total SCF correction =     0.000073
>>>>>      Total force =     0.048789     Total SCF correction =     0.000054
>>>>>      Total force =     0.053071     Total SCF correction =     0.000047
>>>>>      Total force =     0.057755     Total SCF correction =     0.000030
>>>>>      Total force =     0.061205     Total SCF correction =     0.000057
>>>>>      Total force =     0.063732     Total SCF correction =     0.000055
>>>>>      Total force =     0.065333     Total SCF correction =     0.000069
>>>>>      Total force =     0.067697     Total SCF correction =     0.000029
>>>>>      Total force =     0.071297     Total SCF correction =     0.000042
>>>>>      Total force =     0.075401     Total SCF correction =     0.000020
>>>>>      Total force =     0.080403     Total SCF correction =     0.000064
>>>>>      Total force =     0.086012     Total SCF correction =     0.000030
>>>>>      Total force =     0.091511     Total SCF correction =     0.000033
>>>>>
>>>>>
>>>>>
>>>>>           
>> ------------------------------------------------------------------------
>>     
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>>>>>
>>>>>           
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>
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