<div dir="ltr"><div>Hi QE Experts,</div><div><br></div><div>Please know that before sending this question, I have done my best to extensively read the existing body of past forum messages and other QE related learning materials. <br></div><div><br></div><div>I am currently studying NV centers in bulk diamond, and I have a question regarding a single NV0 (charge neutral) center I have made in a 3x3x3 (216) atom supercell of bulk diamond. In this system, we have an odd number of electrons, leaving a single lone electron
(spin-up in this case). Therefore, I expect that my total magnetization should be 1.0
Bohr mag/cell, and I see this consistently in my QE outputs. I am comfortable in thinking that my system is ferromagnetic, based on my deductions from reading the literature. However, I have some discrepancy when it comes to the absolute magnetization, and it is here where my question lies.</div><div><br></div><div>When I fix the
total magnetization to be = 1.0
Bohr mag/cell, and use a fixed occupations scheme, the absolute magnetization for some reason converges to a value of 2.11 Bohr mag/cell. I find this to be strange, since it should be around the value of the total magnetization, which is 1 .0
Bohr mag/cell. What this tells me is that for some reason, perhaps I am converging to some anti-ferromagnetic solution. Then again, I don't know if this is even possible given that I am using fixed occupations.</div><div><br></div><div>Next, when I use occupations = "smearing", ("cold") and set only a guess starting magnetization (do not fix total magnetization), I find that I actually get a value for BOTH the total and absolute magnetization to be around 1.0
Bohr mag/cell, which is more or less what I expect to see, given that I believe that my system is rightfully a simple ferromagnetic system.<br></div><div><br></div><div>So my question is, what the heck is going on in the case of fixed occupations? why am I converging to solution in which the total magnetization is 1.0
Bohr mag/cell, and the absolute magnetization is 2.11
Bohr mag/cell? Is there any apparent misunderstanding I may be having in my analysis? I seek your expertise in this regard. <br></div><div><br></div><div>I have attached my PWscf input and output files. The output file that was used with smearing is labeled "x0.scf_smear.out", and the output file in which fixed occupations were used along with setting tot_magnetization is labeled "x0.scf_fixed.out". The input file is labeled "<a href="http://x0.scf.in">x0.scf.in</a>". To run the calculations with the fixed occupations, I just comment out the smearing part and uncomment the tot_magnetization line. <br></div><div><br></div><div>Thank you for your time in reading my email. I look forward to any suggestions.</div><div><br></div><div>Best,<br></div><div>Brendan A. Smith</div><div>Ph.D candidate at the State University of New York at Buffalo<br></div><div><br></div></div>