<div dir="ltr"><div><div><div>Dear users,<br><br></div>When we calculate the phonon spectrum of a rather obscure mineral, K2Si4O9, at high pressures, we encounter a strange problem.<br><br></div>The unit cell contains 60 atoms, for which the code found two Sym. ops. One is the
identical operator, the other is 180 deg rotation - cart. axis [0,0,1]
plus (0,0,0.5) fractional translation. Using the default 'nosym = .false.' in
the scf input, we found large imaginary frequencies at q=(0,0,1/2),<br>
<br> omega( 1) = -89.679305 [THz] = -2991.379628 [cm-1]<br> omega( 2) = -89.679305 [THz] = -2991.379628 [cm-1]<br> omega( 3) = -88.598203 [THz] = -2955.317953 [cm-1]<br> omega( 4) = -88.598203 [THz] = -2955.317953 [cm-1]<br>
omega( 5) = 2.408244 [THz] = 80.330387 [cm-1]<br> omega( 6) = 2.408244 [THz] = 80.330387 [cm-1]<br> omega( 7) = 2.465075 [THz] = 82.226043 [cm-1]<br> omega( 8) = 2.465075 [THz] = 82.226043 [cm-1] ...<br>
<br></div><div>Searching more stable structures along the presumed
'unstable' modes was in vain, which led us to suspect the above
imaginary frequencies are artifacts. Indeed, by setting the 'nosym =
.true.', we found<br>
<br> omega( 1) = 2.289272 [THz] = 76.361882 [cm-1]<br> omega( 2) = 2.289349 [THz] = 76.364467 [cm-1]<br> omega( 3) = 2.373282 [THz] = 79.164179 [cm-1]<br> omega( 4) = 2.373320 [THz] = 79.165434 [cm-1]<br>
omega( 5) = 2.668095 [THz] = 88.998078 [cm-1]<br> omega( 6) = 2.668166 [THz] = 89.000448 [cm-1]<br> omega( 7) = 2.867070 [THz] = 95.635151 [cm-1]<br> omega( 8) = 2.867215 [THz] = 95.639985 [cm-1]...<br>
<br></div><div>This problem is independent of the pseudopotentials used, and appears in pwscf 4.3.2 as well as the patched 5.0.3.<br><br></div><div>The
relevant input and output files are attached below. To speed up
reproducing the error, the k-point mesh was trimmed to gamma point
only. <br>
<br></div><div>Thank you.<div><div><img src="https://mail.google.com/mail/u/0/images/cleardot.gif"></div></div><span><font color="#888888"></font></span></div>
<span><font color="#888888"><div>Tao Sun<br></div><div>College of Earth Sciences<br></div><div>University of Chinese Academy of Sciences<br></div></font></span></div>