Dear PWSCF users,<br>
I have done a calculation of LaAlO3 recently, using 'vc-relax'
with the contraints that only z-direction is relaxed and x,y directions
are fixed, and in the presence of finite electric field (based on Berry
Phase method). The input file is attached at the end.<br>
However I am very confused with the
results. The equilibrium
lattice constant in z direction is c=0.95*a (a is the lattice constant
in x and y direction). The final ionic polarization is 72.03 a.u.
and
electronic polarization is 4.50 a.u. Then I use the equilibrium unit
cell (c=0.95*a) and just 'relax' the atoms in the presence of the same
electric field. I obtain: ionic polarization is 75.13 a.u. and
electronic polarization is 1.36 a.u. Even more confusing is that if I
use the equilibrium unit cell (c=0.95*a) and put the atom in the
ideal position (i.e. no ionic polarization), the reference ionic
polarization is 73.24 a.u. <br>
Shall I trust the 'vc-relax' calculation in the presence of finite electric field?<br>
Thank you very much.<br>
<br>
Input file reads:<br>
&CONTROL<br>
calculation='vc-relax'<br>
wf_collect=.true.<br>
pseudo_dir = './psp'<br>
outdir='/scratch'<br>
wfcdir='/scratch'<br>
prefix='sLAO-vc'<br>
tprnfor = .true.<br>
tstress = .true.<br>
disk_io='low'<br>
verbosity='high'<br>
dt=80.D0<br>
lelfield=.true.<br>
gdir=3<br>
nppstr=16<br>
nberrycyc=1<br>
/<br>
&SYSTEM<br>
ibrav= 6<br>
celldm(1) = 7.27<br>
celldm(3) = 0.9506<br>
nat= 5<br>
ntyp= 3<br>
ecutwfc = 30.0<br>
ecutrho = 180.0<br>
occupations='fixed'<br>
nosym=.true.<br>
/&ELECTRONS<br>
diagonalization='david'<br>
mixing_beta = 0.7D0<br>
diago_david_ndim = 4<br>
startingwfc='random'<br>
startingpot='atomic'<br>
efield=0.00348<br>
conv_thr = 1.0d-9<br>
/<br>
&IONS<br>
ion_dynamics = 'damp'<br>
phase_space = 'full'<br>
pot_extrapolation = 'second_order'<br>
wfc_extrapolation = 'second_order'<br>
/<br>
&CELL<br>
cell_dynamics = 'damp-w'<br>
cell_dofree = 'z'<br>
/<br>
ATOMIC_SPECIES<br>
La 138.91 057-La-ca-nsp-hanghui.uspp.format.UPF<br>
Al 26.98 013-Al-ca--hanghui.uspp.format.UPF<br>
O 16.00 008-O-ca--vgrp.uspp.format.UPF<br>
ATOMIC_POSITIONS crystal<br>
La 0.00 0.00 0.00<br>
Al 0.50 0.50 0.50<br>
O 0.50 0.50 0.00<br>
O 0.00 0.50 0.50<br>
O 0.50 0.00 0.50<br>
K_POINTS crystal<br>
256<br>
(The k points are omitted here)<br>
<br>
Hanghui Chen<br>
Department of Physics <br>
Yale University<br>
<br>
<br>